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Preparation and characterization of Cf/Pollucite composites through geopolymer precursors
Affiliation:1. Additive Manufacturing Institute, College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen, Gaungdong, 518110, China;2. Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province, College of Optoelectronic Engineering, Shenzhen University, Shenzhen, Gaungdong, 518110, China;3. Institute for Advanced Ceramics, School of Materials Science and Engineering, Harbin Institute of Technology, Harbin, Heilongjiang, 150080, China
Abstract:Continuous carbon-fibre-reinforced Cs-geopolymer composite (Cf/CsGP) were prepared, and its in-situ conversion was investigated during high-temperature treatments. The effect of treatment temperature on the thermal evolution process and mechanical properties of the resulting products were systematically evaluated. The results indicated that the crystallization temperature of Cf/CsGP composite was considerably delayed because the amorphous structure of carbon fibres was not conducive as a nucleation substrate for pollucite derived from the CsGP matrix. Moreover, the integrity of the corresponding resulting products derived from the Cf/CsGP composite were damaged due to thermal shrinkage that occurred during the high-temperature treatment process. When treatment temperature was ≤1200oC, the mechanical properties of the corresponding products exhibited an upward trend, which was ascribed to the improvement of the densification degree of the resulting composite and well interface-bonding state between carbon fibres and pollucite. However, the mechanical properties of the resulting composites decreased with the treatment temperature continued increased from 1200 to 1400oC. This phenomenon was attributed to the impairment of fibre properties caused by interfacial reactions.
Keywords:Geopolymer composite  Carbon fibre  Pollucite  Microstructure  Mechanical property
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