Phase Disequilibrium in the Course of an Exothermic Reaction Accompanied by Liquid Evaporation in a Catalytic Trickle-Bed Reactor |
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Authors: | Shigarov A B Kuzin N A Kirillov V A |
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Affiliation: | (1) Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, pr. akademika Lavrent'eva 5, Novosibirsk, 630090, Russia |
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Abstract: | -Methylstyrene hydrogenation in a fixed catalyst bed is studied experimentally and theoretically for a cocurrent downflow of the gas and liquid. Gas-phase hydrogenation on dry catalyst granules disturbs the liquid–vapor phase equilibrium. A dimensionless parameter related to the Raoult–Dalton law for a liquid–vapor mixture is suggested to characterize phase disequilibrium in the system. |
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