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From “100%” Utilization of MAX/MXene to Direct Engineering of Wearable,Multifunctional E-Textiles in Extreme Environments
Authors:Bin Li  Na Wu  Qilei Wu  Yunfei Yang  Fei Pan  Wei Liu  Jiurong Liu  Zhihui Zeng
Affiliation:1. Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials (Ministry of Education), School of Materials Science and Engineering, Shandong University, Jinan, 250061 P. R. China;2. Department of Mechanical Engineering, The Hong Kong Polytechnic University, Kowloon, Hong Kong, 999077 P. R. China;3. Science and Technology on Electromagnetic Compatibility Laboratory, China Ship Development and Design Centre, Wuhan, 430064 P. R. China;4. Department of Chemistry, University of Basel, Basel, CH-4058 Switzerland;5. State Key Laboratory of Crystal Materials, Institute of Crystal Materials, Shandong University, Jinan, 250100 P. R. China

Shenzhen Research Institute of Shandong University, Shandong University, Shenzhen, 518057 P. R. China

Abstract:Transition metal carbides/nitrides (MXenes) show great potential for preparing wearable, flexible multifunctional e-textiles due to the exceptional electrical and mechanical properties and easy processing in aqueous medium. At present, MXene-based e-textiles face challenges including high production costs, low utilization of precursor titanium aluminum carbide (MAX), poor durability in extreme environments, and the inability to achieve a balance between large-scale fabrication and high performance. Here, this work proposes a “100%” utilization of MAX/MXene strategy to produce additive-free conductive inks with controllable viscosity, subsequently enabling an accessible, scalable direct-blade-coating followed by chemical cross-linking approach for creating wearable, high-performance, multifunctional MXene-based e-textiles that perform in extreme conditions. The structural design provides integrated multifunctionality involving controllable and exceptional electromagnetic interference (EMI) shielding within an ultrabroadband frequency range, visual electrothermal conversion, electrothermal deicing, remarkable visual photothermal, and antibacterial performance. This work employs a fabrication process that is simple, cost-effective, and scalable, presenting a novel “100% efficiency” and “waste-to-wealth” strategy to manufacture robust, durable, multifunctional e-textiles. This approach provides exciting potential for the next generation of wearable electronics, EMI compatibility, visual heating, thermotherapy, antibacterial treatments, deicing, defense, and aerospace applications.
Keywords:e-textiles  flexible  multifunctionality  MXenes  wearables
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