Device-Level Optimization of n-Type Mg3(Sb,Bi)2-Based Thermoelectric Modules toward Applications: A Perspective |
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Authors: | Congcong Xu Zhongxin Liang Shaowei Song Zhifeng Ren |
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Affiliation: | Department of Physics and Texas Center for Superconductivity at the University of Houston (TcSUH), University of Houston, Houston, TX, 77204 USA |
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Abstract: | In recent decades, improvements in thermoelectric material performance have made it more practical to generate electricity from waste heat and to use solid-state devices for refrigeration. However, despite the development of successful strategies to enhance the figure-of-merit zT, optimizing devices for large-scale applications remains challenging. High zT values do not guarantee excellent device performance, and maintaining high zT over a wide temperature range is difficult. Thus, device-level structural optimization is crucial for maximizing overall energy conversion efficiency. Proper interfacial and structure design strategies, including contact layer selection, multi-stage optimization, and size matching for the n- and p-type thermoelectric legs, are necessary for advancing device performance. Additionally, thermal stability issues, device assembly techniques, mechanical properties, and manufacturing costs are crucial considerations for large-scale applications. To achieve actual applications, the thermoelectric community must look beyond simply aiming for high zT values. This article focuses on modules based on n-type Mg3(Sb, Bi)2, one of the most promising commercially available thermoelectric materials, and discusses the influence of various parameters on the modules and on the corresponding device-level optimization strategies. |
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Keywords: | device optimizations Mg3(Sb Bi)2 thermoelectrics cooling thermoelectrics power generation |
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