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Tandem organic light-emitting diodes with buffer- modified C60/pentacene as charge generation layer
Authors:WANG Zhen  ZHENG Xin  LIU Fei  WANG Pei  GAN Lin  WANG Jing-jing
Affiliation:College of Optoelectronic Engineering, Chongqing University of Posts and Telecommunications, Chongqing 400065, China,College of Optoelectronic Engineering, Chongqing University of Posts and Telecommunications, Chongqing 400065, China,College of Optoelectronic Engineering, Chongqing University of Posts and Telecommunications, Chongqing 400065, China,College of Optoelectronic Engineering, Chongqing University of Posts and Telecommunications, Chongqing 400065, China,College of Optoelectronic Engineering, Chongqing University of Posts and Telecommunications, Chongqing 400065, China and College of Optoelectronic Engineering, Chongqing University of Posts and Telecommunications, Chongqing 400065, China
Abstract:Buffer-modified C60/pentacene as charge generation layer (CGL) is investigated to achieve effective performance of charge generation. Undoped green electroluminescent tandem organic light-emitting diodes (OLEDs) with multiple identical emissive units and using buffer-modified C60/pentacene organic semiconductor heterojunction (OHJ) as CGL are demonstrated to exhibit better current density and brightness, compared with conventional single-unit devices. The current density and brightness both can be significantly improved with increasing the thickness of Al. However, excessive thickness of Al seriously decreases the transmittance of films and damages the interface. As a result, the maximum current efficiency of 1.43 cd.A-1 at 30 mA.cm-2 can be achieved for tandem OLEDs with optimal thickness of Al. These results clearly demonstrate that Cs2CO3/Al is an effective buffer for C60/pentacene-based tandem OLEDs.
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