Abstract: | This study introduces carbon nanotube buckypaper (CNTBP) into the easily fractured sites of [0°]16 and [0°/90°]4S composite laminates, and comparatively explores how the CNTBP affects the flexural properties of the laminates at 25, ?15, and ?55 °C. Compared to the base [0°]16 and [0°/90°]4S laminates at the same temperature, improvements of the flexural strengths in the order of 4.0–15.3% and 6.5–31.0% are respectively obtained from the corresponding CNTBP‐reinforced [0°]16 and [0°/90°]4S laminates. Importantly, the lower the temperature is, the higher the strength improves. In fact, the CNTBP has little effect on the flexural moduli of the studied laminates, although there is an increasing trend with decreased temperature. Moreover, the introduced CNTBP would significantly change the fracture mechanism of the laminates at low temperature. The present work reveals that the CNTBP exhibits more positive reinforcing capability to the polymer matrix‐based composite laminates at relatively low temperatures. |