Environmentally friendly alcohol oxidation using heterogeneous catalyst in the presence of air at room temperature |
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| Affiliation: | 1. Center for Composite Materials and Structures, Harbin Institute of Technology, Harbin 150001, China;2. Key Laboratory of Micro-systems and Micro-structures Manufacturing, Ministry of Education, China;3. Center of Analysis Measurement, Harbin Institute of Technology, Harbin 150001, China;1. Engelhardt Institute of Molecular Biology, Russian Academy of Sciences, Moscow 119991, Vavilov Street 32, Russia;2. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Moscow 119991, Vavilov Street 28, Russia;3. Department of Chemistry and Biochemistry and Molecular Biology, University of Georgia, Athens, GA 30602, USA;4. Department of Biological Sciences, State University of New York at Buffalo, Buffalo, NY 14260, USA;1. Department of Chemistry, College of Sciences, Shanghai University, Shanghai 200444, China;2. Department of Criminal Investigation, Sichuan Police College, Luzhou 646000, China;1. Division of Physical Science and Engineering, King Abdullah University of Science and Technology, Thuwal 23955-6900, Saudi Arabia;2. Key Laboratory of Advanced Textile Materials & Manufacturing Technology, Ministry of Education, Zhejiang Sci-Tech University, Hangzhou, Zhejiang 310018, People’s Republic of China;3. Eco-Dyeing and Finishing Engineering Research Center, Ministry of Zhejiang Sci-Tech University, Hangzhou, Zhejiang 310018, People’s Republic of China;4. National Base for International Science and Technology Cooperation in Textiles and Consumer-Goods Chemistry, Zhejiang Sci-Tech University, Hangzhou, Zhejiang 310018, People’s Republic of China;5. CAS Key Laboratory of Low-carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201210, People’s Republic of China |
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| Abstract: | Various types of alcohols oxidation can be achieved using air as a sole oxidant at room temperature without any other additives. From the results of Ru K-edge XAFS and XPS characterizations, MnFe1.5Ru0.35Cu0.15O4 catalyst with possibly coordinatively unsaturation of the isolated RuO species as active sites is an efficient heterogeneous catalyst and can be reused. Besides, the workup procedure is extremely simple. |
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