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One-pot solvothermal synthesis of 1D plasmonic TiO2@Ag nanorods with enhanced visible-light photocatalytic performance
Affiliation:1. School of Chemistry and Chemical Engineering, Institute of Physical Chemistry, Lingnan Normal University, Zhanjiang, 524048, PR China;2. Centre for Clean Environment and Energy, School of Environment and Science, Gold Coast, Griffith University, QLD, 4222, Australia;3. State Key Laboratory of Resources and Environmental Information System, Institute of Geographic Sciences and Natural Resources Research of Chinese Academy of Sciences, Beijing, 100101, PR China;1. College of Science, Northeast Agricultural University, Harbin, Heilongjiang, 150030 PR China;2. Department of Chemistry, College of Science, Northeast Forestry University, Harbin 150040, PR China;1. School of Chemical and Biological Engineering, Lanzhou Jiaotong University, Lanzhou 730070, China;2. Department of Materials and Environmental Chemistry (MMK), Stockholm University, Stockholm 10691, Sweden;3. Key Laboratory of Eco-Environment-Related Polymer Materials, Ministry of Education of China, Key Laboratory of Gansu Polymer Materials, College of Chemistry and Chemical Engineering, Northwest Normal University, Lanzhou 730070, China;1. Skolkovo Institute of Science and Technology, 3 Nobel St, 121205 Moscow, Russian Federation;2. Yuri Gagarin State Technical University, 410054 Saratov, 77 Polytechnicheskaya St, Russian Federation;3. Saratov Branch of Kotelnikov Institute of Radioengineering and Electronics of RAS, 410019 Saratov, 38 Zelenaya St, Russian Federation;4. Systems for Microscopy and Analysis, 121353 Moscow, Skolkovskoe sh. 45, off. 20, Russian Federation;5. Korea Institute of Science and Technology Europe, Campus E7 1, 66123 Saarbrücken, Germany;6. Saarland University, 3 Campus Dudweiler Zeile, 66125 Saarbrücken, Germany;7. Aalto University, Puumiehenkuja, 00076 Aalto, Finland;1. College of Mechanical Engineering, Yangzhou University, Yangzhou 225127, China;2. School of Materials Science and Engineering, Jiangsu Key Laboratory of Advanced Metallic Materials, Southeast University, Nanjing 211189, China;3. College of Materials Science and Engineering, Nanjing Tech University, 5 Xinmofan Road, Nanjing 210009, China;1. Tsinghua University – Zhang Jiagang Joint Institute for Hydrogen Energy and Lithium-Ion Battery Technology, INET, Tsinghua University, Beijing 100084, PR China;2. Collaborative Innovation Center for Advanced Nuclear Energy Technology, INET, Tsinghua University, Beijing 100084, PR China;3. Beijing Key Laboratory of Radioactive Waste Treatment, INET, Tsinghua University, Beijing 100084, PR China
Abstract:A plasmonic photocatalyst is designed and synthesized by coating TiO2 nanoparticles onto the surface of Ag nanorods (Ag NRs), namely one-dimensional TiO2@Ag NRs photocatalyst. Materials characterizations suggest that the as-prepared catalysts consist of a uniform and high crystalline anatase nanocrystals and highly conductive Ag nanorod. It delivers remarkable visible-light photocatalytic performance in simultaneous H2 evolution and decomposition of methyl orange (MO) due to the synergetic effects of plasmonic resonance under visible light irradiation, a matched heterojunction, high surface area and large conductivity.
Keywords:Semiconductor  Heterostructures  Plasmon resonance  Ag nanorods
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