Bimetallic metal-organic framework derived electrocatalyst for efficient overall water splitting |
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Affiliation: | 1. Centre for Technology in Water and Wastewater, School of Civil and Environmental Engineering, University of Technology Sydney, NSW, 2007, Australia;2. Center for Clean Energy Technology, School of Mathematical and Physical Science, Faculty of Science, University of Technology Sydney, NSW, 2007, Australia;1. School of Chemical Engineering and Technology, North University of China, Taiyuan 030051, People’s Republic of China;2. School of Environment and Safety, North University of China, Taiyuan 030051, People’s Republic of China;3. School of Science, North University of China, Taiyuan 030051, People’s Republic of China |
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Abstract: | The development of bifunctional catalysts that can be applied to both hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) is widely regarded as a key factor in the production of sustainable hydrogen fuel by electrochemical water splitting. In this work, we present a high-performance electrocatalyst based on nickel-cobalt metal-organic frameworks for overall water splitting. The as-obtained catalyst shows low overpotential to reaches the current density of 10 mA cm?2 with 249 mV for OER and 143 mV for HER in alkaline media, respectively. More importantly, when the electrolyzer was assembled with the as-prepared catalyst as anode and cathode simultaneously, it demonstrates excellent activity just applies a potential of 1.68 V to achieve 10 mA cm?2 current density for overall water splitting. |
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Keywords: | Hydrogen evolution reaction Oxygen evolution reaction Overall water splitting Electrocatalyst |
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