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Criterion for extinction of CO oxidation in a catalytic monolith
Authors:Vladimir P. Zhdanov
Affiliation:1. Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian, 116023, China
Abstract:The extinction of CO oxidation occurring on the Pt catalyst in a monolithic reactor depends on the interplay of the reaction kinetics and mass and heat transfer. In particular, it may be related to a first-order kinetic phase transition from the high-reactive regime to the low-reactive regime. For this scenario, we obtain the criterion for extinction.
Keywords:extinction  ignition  kinetic phase transitions  mass-transport limitations  monolithic catalytic reactor  CO oxidation  Pt
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