Electrical characterizations of PZT ceramics in large frequency and temperature ranges |
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Authors: | D. Fasquelle J.C. Carru |
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Affiliation: | aLEMCEL, Université du Littoral Côte d’Opale, 50 rue Ferdinand Buisson, B.P. 717, 62228 Calais Cedex, France |
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Abstract: | Electrical properties of PbZr0.75Ti0.25O3 ceramics have been characterized. The measurements have been made in frequency ranging from 20 to 2.109 Hz and between 20 and 730 °C for low and medium frequencies. Typically at room temperature, the dielectric constant ′ is higher than 500 at 1 MHz whereas the loss tangent is close to 0.01. From ′(T) measurements, the Curie temperature of our sample has been determined at 320 °C. In the paraelectric state, ′(T) follows the empirical Curie–Weiss law near the phase transition which is of second order type. The increase of ′ observed at high temperatures and low frequencies in the paraelectric state are explained: this abnormal behavior is due to the migation of oxygen ions towards the electrodes, creating an additional non-ferroelectric interface which generates a Maxwell–Wagner effect. |
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Keywords: | Dielectric properties Electrical conductivity Phase transition PZT |
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