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Tap Reactor for Temporally and Spatially Resolved Analysis of the CO2 Methanation Reaction
Authors:Timo Engl  Moritz Langer  Prof. Dr.-Ing. Hannsjörg Freund  Dr.-Ing. Michael Rubin  Prof. Dr.-Ing. Roland Dittmeyer
Affiliation:1. Karlsruhe Institute of Technology, Institute for Micro Process Engineering (IMVT), Hermann-von-Helmholtz-Platz 1, 76344 Eggenstein-Leopoldshafen, Germany;2. TU Dortmund University, Institute of Reaction Engineering and Catalysis (REC), Emil-Figge-Straße 66, 44227 Dortmund, Germany
Abstract:Chemical energy carriers produced according to power-to-X concepts will play a crucial role in the future energy system. Here, CO2 methanation is described as one promising route. However, transient operating conditions and the resulting effects on catalyst stability are to be considered. In this contribution, a tap reactor for spatially and temporally resolved analysis of the methanation reaction is presented. The Ni catalyst investigated was implemented as coating. Reaction data as a function of time and reactor coordinate under various operating conditions are presented and discussed. A comparison with simulation data validates the presented tap reactor concept.
Keywords:Catalyst coatings  CO2 methanation  Spatially and temporally resolved analysis  Tap reactors  Transient operation
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