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Crystal growth and scintillation properties of Nd-doped Lu3Al5O12 single crystals with different Nd concentrations
Authors:Makoto Sugiyama  Yutaka FujimotoTakayuki Yanagida  Yuui YokotaJan Pejchal  Yuki FuruyaHidehiko Tanaka  Akira Yoshikawa
Affiliation:a Institute of Multidisciplinary Research for Advanced Materials, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai, Miyagi 980-8577, Japan
b Institute of Physics AS CR, Cukrovarnicka 10, Prague 16253, Czech Republic
c New Industry Creation Hatchery Center (NICHe), 6-6-10 Aoba, Aramaki, Aoba-ku, Sendai, Miyagi 980-8579, Japan
Abstract:Nd 0.1%, 0.5%, 1% and 3% doped Lu3Al5O12 (Nd:LuAG) single crystals were grown in the nitrogen atmosphere by the micro-pulling down (μ-PD) method. The grown crystals had a single-phase confirmed by powder XRD analysis. In absorption spectra, some weak absorption lines due to Nd3+ 4f-4f transitions were observed and their intensity increased with the increase of Nd concentration. When excited by 241Am α-ray, a broad emission peak due to defects in the host lattice at 320 nm and some sharp lines due to Nd3+ 4f-4f transitions at wavelength longer than 400 nm were observed. The decay time profiles of Nd:LuAG under γ-ray excitation were well approximated by two exponential function of 340-760 ns and 3-5 μs for each sample. By pulse height measurement using 137Cs, Nd 0.5%:LuAG showed the highest light yield of 7600 ± 760 photons/MeV.
Keywords:LuAG  Single crystal  Scintillator  Nd3+
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