Polar nano-clusters in nominally paraelectric ceramics demonstrating high microwave tunability for wireless communication |
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Affiliation: | 1. School of Electronic Engineering and Computer Science, Queen Mary University of London, Mile End Road, London E1 4NS, UK;2. School of Biological and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK;3. School of Engineering and Materials Science, Queen Mary University of London, Mile End Road, London E1 4NS, UK;4. Institute of Materials Research, Slovak Academy of Sciences, Watsonova 47, 04001 Kosice, Slovakia |
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Abstract: | Dielectric materials, with high tunability at microwave frequencies, are key components in the design of microwave communication systems. Dense Ba0.6Sr0.4TiO3 (BST) ceramics, with different grain sizes, were prepared in order to optimise the dielectric tunability via polar nano cluster effects. Dielectric permittivity and loss measurements were performed at both high and low frequencies and were supported by results from X-ray powder diffraction, scanning and transmission electron microscopies, Raman spectroscopy and piezoresponse force microscopy. The concentration of polar nano clusters, whose sizes are found to be in the range 20–50 nm, and the dielectric tunability increase with increasing grain size. A novel method for measurement of the microwave tunability in bulk dielectrics is presented. The highest tunability of 32 % is achieved in ceramics with an average grain size of 10 μm. The tunability of BST ceramics with applied DC field is demonstrated in a prototype small resonant antenna. |
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Keywords: | Microwave Dielectric Tunability Polarization Ceramics |
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