Probing time-resolved emission in laser-driven electron-multirescattering in a high-order harmonic generation |
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| Authors: | Peng-Cheng Li Chun-Xiao Li Xiong-Yuan Lei Yae-Lin Sheu Xiao-Xin Zhou Shih-I Chu |
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| Affiliation: | 1. College of Physics and Electronic Engineering, Northwest Normal University, Lanzhou, People’s Republic of China;2. Department of Physics, National Taiwan University, Taipei, Taiwan;3. Department of Chemistry, University of Kansas, Lawrence, USA |
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| Abstract: | We present an ab initio study of quantitative extraction of the time–frequency spectra of multiple rescattering processes of the electrons driven by the mid-infrared laser field in a high-order harmonic generation (HHG). The HHG is calculated by solving the three-dimensional time-dependent Schrödinger equation by means of the time-dependent generalized pseudospectral method. We extend a synchrosqueezed transform (SST) technique to extract the individual contributions of multiple rescattering processes in HHG. Combining with an extended semiclassical analysis and the SST time–frequency spectrum, the role of quantum trajectories in multiple rescattering processes in HHG is clarified. We find that the SST allows us to distinguish the individual contribution of multiple rescattering processes in HHG and show the details of the spectral and temporal fine structures of the HHG, which provides an important tool for a deep understanding to the dynamics of multiple rescattering processes in HHG. |
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| Keywords: | High-order harmonic generation intense laser field time–frequency analysis multiple rescattering processes time-dependent Schrödinger equation |
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