Experience in long-term neutron dose equivalent measurements using etched track detectors with (n,alpha) converters in moderators

Etched track Makrofol detectors combined with Kodak BN-1 boron (n,alpha) converters were used inside a 30 cm diameter polyethylene (PE) sphere for the measurement of the neutron ambient dose equivalent. We found unexpectedly high values for the neutron dose equivalent of about 250 microSv instead of 25 microSv for 3 months' exposure in the natural environment. Results from such detectors etched in the authors' labortories revealed that the tracks could only be induced by spontaneous particle emission from the converter. This was confirmed by track diameter analysis and additional special etching of deeper detector layers. Eight surface barrier detectors were used simultaneosly for several days to measure the alpha spectra of the converters. The overall count rate in the energy range 2.5-7.5 MeV was 10 alpha particles d(-1) x cm(-2) for most of the converters and about 10 times less than this for some of them. To identify the nuclides responsible for alpha emission within the converters, gamma spectra of converters were measured for 8 days using a highly sensitive low-background gamma spectrometry system The spectra clearly indicated a small contamination (10 +/- 3 mBq) of the converter foils with 225Ra (T(1/2) = 5.7 y) typically originating from 232Th.