Compact and vertically-aligned ZnO nanorod thin films by the low-temperature solution method |
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Authors: | Chu-Chi Ting Chang-Hung Li Chih-You Kuo Chia-Chen Hsu Hsiang-Chen Wang Ming-Hsun Yang |
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Affiliation: | Graduate Institute of Opto-Mechatronics Engineering, National Chung Cheng University, 168 University Rd., Min-Hsiung, Chia-Yi, Taiwan ROC |
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Abstract: | Highly c-axis-oriented ZnO nanorod thin films were obtained on silica glass substrates by a simple solution-growth technique. The most compact and vertically-aligned ZnO nanorod thin film with the thickness of ∼ 800 nm and average hexagonal grain size of ∼ 200 nm exhibits the average visible transmittance 85%, refractive index 1.74, packing density 0.84, and energy band gap 3.31 eV, and it was fabricated under the optimum parameters: 0.05 M, 75 °C, 6 h, multiple-stepwise, and ZnO seed layer with an average grain size of ∼ 20 nm. The photoluminescence spectrum indicates that the densest ZnO nanorod thin film possesses lots of oxygen vacancies and interstitials. As we demonstrate here, the solution-growth technique was used to produce high-quality and dense ZnO nanorod thin films, and is an easily controlled, low-temperature, low-cost, and large-scale process for the fabrication of optical-grade thin films. |
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Keywords: | Zinc oxide Nanorods Packing density Chemical solution deposition Transmittance Photoluminescence Scanning electron microscopy |
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