Methane aromatization over Mo/H-ZSM-5: on the reaction pathway |
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Authors: | P. Mériaudeau Vu Thi Thu Ha Le Van Tiep |
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Affiliation: | (1) IRC/CNRS, 2, avenue A. Einstein, 69626 Villeurbanne, France |
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Abstract: | Rates of benzene formation on Mo/HZSM-5, H-ZSM-5 and Mo/SiO2 were measured with different reactants: methane, mixture of C2H4/H2/N2 and mixture of C2H2/H2/N2. Since the rate of benzene formation starting from C2H4/H2/N2 is higher on Mo/H-ZSM-5 compared to H-ZSM-5 it is concluded that the aromatization of methane on Mo/H-ZSM-5 is not going via ethylene which is aromatized over acid sites. Another reaction pathway is proposed. This revised version was published online in July 2006 with corrections to the Cover Date. |
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Keywords: | methane aromatization ethylene aromatization acetylene aromatization |
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