Correlation relations for estimating the content of plutonium isotopes in fallout due to the Chernobyl accident

The possibility of determining the total α activity A(^239,240Pu) of ²³⁹Pu + ²⁴⁰Pu according to the γ radiation of ¹⁰³Ru and ¹⁰⁶Ru is examined. The statistical properties of the experimental ratios of the activities ρ = A(¹⁰⁶Ru)/A(¹⁰³Ru) are investigated. The distribution of the experimental ratios is similar to the theoretical ratios for fuel and close to a Gaussian distribution with average value 〈p〉 = 0.22 and standard deviation Δ ∼ 0.06. This ratio is used to obtain a relation for estimating A(^239,240Pu) from the γ activity A(¹⁰³Ru). A theoretical analysis is made of the experimental data for the southern raions of Gomel oblast. It is shown that given a good statistical sample of measurements of the γ activity of ¹⁰³Ru it is possible to estimate the average value of the γ activity A(^239,240Pu) and with probability 0.95 the interval of the possible values of this activity. __________ Translated from Atomnaya énergiya, Vol. 103, No. 4, pp. 255–259, October, 2007.