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Nonlinear model reconstruction by frequency and amplitude response for a heterogeneous binary reaction in a chemostat
Authors:William B. Zimmerman
Affiliation:Department of Chemical and Process Engineering, University of Sheffield, Newcastle Street, Sheffield S1 3JD, UK
Abstract:Here we present an analysis of a binary heterogeneous reaction in a chemostat for the particular case of reagents with unequal mass transfer coefficients. For fast irreversible kinetics, there are two potential steady states—the dispersed phase is preferentially populated by one reagent and essentially depleted of the other. The selection of which steady state occurs depends on the operating parameter which is the concentration ratio σ of the slower (B) to the faster (A) transferring reagent in the feed stream. The demarcation between these operating regimes is the critical value of this ratio:
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Keywords:Nonlinear dynamics   Data assimilation   Kinetics models reconstruction   Frequency response   Heterogeneous reaction engineering   Chemostat
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