A flexible apparatus for attosecond photoelectron spectroscopy of solids and surfaces |
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Authors: | Magerl E Neppl S Cavalieri A L Bothschafter E M Stanislawski M Uphues Th Hofstetter M Kleineberg U Barth J V Menzel D Krausz F Ernstorfer R Kienberger R Feulner P |
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Affiliation: | Max-Planck-Institut fu?r Quantenoptik, Hans-Kopfermann-Stra?e 1, 85748 Garching, Germany. |
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Abstract: | We describe an apparatus for attosecond photoelectron spectroscopy of solids and surfaces, which combines the generation of isolated attosecond extreme-ultraviolet (XUV) laser pulses by high harmonic generation in gases with time-resolved photoelectron detection and surface science techniques in an ultrahigh vacuum environment. This versatile setup provides isolated attosecond pulses with photon energies of up to 140 eV and few-cycle near infrared pulses for studying ultrafast electron dynamics in a large variety of surfaces and interfaces. The samples can be prepared and characterized on an atomic scale in a dedicated flexible surface science end station. The extensive possibilities offered by this apparatus are demonstrated by applying attosecond XUV pulses with a central photon energy of ~125 eV in an attosecond streaking experiment of a xenon multilayer grown on a Re(0001) substrate. |
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