In-pile Xe diffusion coefficient in UO2 determined from the modeling of intragranular bubble growth and destruction under irradiation |
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Authors: | K Govers S Lemehov |
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Affiliation: | a Service de Métrologie Nucléaire (CP 165/84), Université Libre de Bruxelles, 50 Avenue F.D. Roosevelt, B-1050 Bruxelles, Belgium b Institute of Nuclear Materials Science, SCK·CEN, Boeretang 200, B-2400 Mol, Belgium |
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Abstract: | Intragranular bubbles grow in the nuclear fuel by diffusion and precipitation of fission gases, mainly xenon; and are ultimately destroyed, under irradiation, by fission fragments. This article will attempt to determine the in-pile bubble distributions taking into account the evolution of the concentration profile around a bubble during its growth and the destruction process by fission fragments. From these distributions a relation between the bubble mean radius and the diffusion coefficient of xenon can be established, allowing the determination, from experimental measurements of intragranular bubble sizes, of the in-pile Xe diffusion coefficient in UO2. The estimated activation energy (0.9 eV) is about one order of magnitude lower than the widely used value of 3.9 eV determined from out-of-pile experiments. This effect can be attributed to the presence of point defects created by the irradiation. |
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Keywords: | 61 72 Ji 61 72 Qq 61 80 &minus x 66 10 Cb 66 30 &minus h 66 30 Jt |
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