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Enhancing the Quantum Anomalous Hall Effect by Magnetic Codoping in a Topological Insulator
Authors:Yunbo Ou  Chang Liu  Gaoyuan Jiang  Yang Feng  Dongyang Zhao  Weixiong Wu  Xiao‐Xiao Wang  Wei Li  Canli Song  Li‐Li Wang  Wenbo Wang  Weida Wu  Yayu Wang  Ke He  Xu‐Cun Ma  Qi‐Kun Xue
Affiliation:1. State Key Laboratory of Low Dimensional Quantum Physics, Department of Physics, Tsinghua University, Beijing, China;2. Collaborative Innovation Center of Quantum Matter, Beijing, P. R. China;3. Department of Physics and Astronomy, School of Arts and Sciences, Rutgers University, Piscataway, NJ, USA
Abstract:The quantum anomalous Hall (QAH) effect, which has been realized in magnetic topological insulators (TIs), is the key to applications of dissipationless quantum Hall edge states in electronic devices. However, investigations and utilizations of the QAH effect are limited by the ultralow temperatures needed to reach full quantization—usually below 100 mK in either Cr‐ or V‐doped (Bi,Sb)2Te3 of the two experimentally confirmed QAH materials. Here it is shown that by codoping Cr and V magnetic elements in (Bi,Sb)2Te3 TI, the temperature of the QAH effect can be significantly increased such that full quantization is achieved at 300 mK, and zero‐field Hall resistance of 0.97 h/e2 is observed at 1.5 K. A systematic transport study of the codoped (Bi,Sb)2Te3 films with varied Cr/V ratios reveals that magnetic codoping improves the homogeneity of ferromagnetism and modulates the surface band structure. This work demonstrates magnetic codoping to be an effective strategy for achieving high‐temperature QAH effect in TIs.
Keywords:ferromagnetic homogeneity  magnetic codoping  quantum anomalous Hall effect  topological insulators
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