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International Symposium on Isotope Separation and Chemical Exchange Uranium Enrichment
Abstract:From the viewpoint of nuclear criticality safety, it is important to comprehend the reactivity of fuel solutions induced by oscillatory movements such as earthquakes. This paper intends to figure out the reactivity of a fuel solution system with a free surface formed by oscillation by evaluating the fluctuation of the neutron multiplication factor (k eff ) obtained from a static calculation. To fulfill this intension, criticality calculations with reflecting fluid calculation results have been carried out. In the fluid calculations, the finite volume method and the volume of fluid (VOF) method have been applied in tracking the free surface formed by oscillation. The continuous energy Monte Carlo calculation method has been applied in the criticality calculations. As a result, it has been found that the variation patterns of the k eff and those of the shape of fuel solutions are classified according to oscillation frequency and the ratio of solution height to the width of the tank (H/L). If a sloshing motion is generated, the k eff fluctuates widely and has a threshold, with which we can classify the fluctuation type of the k eff , despite the kind of reflector. If H/L is above the threshold, i.e., H/L =0.4, the k eff fluctuates to a value below that obtained in the resting state. On the contrary, if H/L is below the threshold, the k eff fluctuates to a value above that obtained in the resting state. This result implies the criticality calculation for a fuel solution with a free surface using the Monte Carlo method may give a slightly smaller threshold than using other approaches.
Keywords:cobalt 60  strontium 90  cesium 137  leaching test  low-level radioactive wastes  plastic-based waste form  leaching ratio  seawater  water  soils  radioactivity
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