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Measurements of Average Cross Section for 232Th(n, 2n)231Th Reaction to Neutrons with Fission-Type Reactor Spectrum and of Gamma-Ray Intensities of 231Th
Abstract:The average cross section for the 232Th(n, 2n)231Th reaction to neutrons with the energy spectrum close to that of fission neutrons was obtained in the core of the Kyoto University Reactor, KUR. The value obtained was 12.5±0.84 mb. This value agrees satisfactorily with Phillips' and with the calculated value obtained with the cross section in the U-K library and the Maxwellian fission neutron spectrum given by Leachman. A somewhat poorer agreement is seen with the calculated value obtained from Butler & Santry's cross section and Leachman's spectrum. The discrepancy amounts to 24 and to 39% respectively, for the average cross sections calculated with these two excitation functions and the fission neutron spectrum given by McElroy.

By making use of a Ge(Li) counter whose photopeak efficiency had been carefully calibrated, the absolute intensities were determined for eleven photopeaks observed on the γ-ray spectrum emitted by 231Th.
Keywords:praseodymium 143  cerium  cation-exchange separation  cerium carbonates  thermal decomposition
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