Heat transport limitations and reaction scheme of partial oxidation of methane to synthesis gas over supported rhodium catalysts |
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| Authors: | Yiannis Boucouvalas Zhaolong Zhang Xenophon E. Verykios |
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| Affiliation: | (1) Institute of Chemical Engineering and High Temperature Chemical Processes, Department of Chemical Engineering, University of Patras, GR-26500 Patras, Greece |
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| Abstract: | The partial oxidation of methane to synthesis gas over supported Rh catalysts is investigated, paying particular attention to removing heat transport limitations and identifying the reaction conditions within the kinetic-controlling regime. The results obtained suggest that the reaction follows the sequence of total oxidation to CO2 and H2O, followed by reforming reactions to synthesis gas. |
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| Keywords: | methane oxidation synthesis gas rhodium catalyst heat transport |
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