Hierarchically porous carbon derived from renewable Chingma Abutilon Seeds for high-energy supercapacitors |
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Authors: | Mutian Ma Yuanhao Wang Yongli Chen Fengzhi Tan Yafeng Cao Weijie Cai |
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Affiliation: | School of Light Industry and Chemical Engineering, Dalian Polytechnic University, Dalian 116034, Liaoning, China |
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Abstract: | The cost-effectively biomass-derived porous carbon is highly promising for usage in electrochemical energy storage as the electrode materials. Herein, a series of hierarchically porous carbons with biomass Chingma Abutilon Seeds as the renewable precursor were synthesized via KOH activation and high-temperature carbonization technique. The resulting carbon material possessed an interconnected structure, high specific surface area (120–3566 m2 g?1), hierarchical pores as well as the heteroatom-substituted functional groups. Based on the synergistic effect of the above-mentioned merits, the optimized material exhibited the remarkably electrochemical performance with high specific capacitance (389 F g?1 at 0.5 A g?1) and excellent rate stability (72% capacitance retention at 20 A g?1) in the three-electrode configuration. More significantly, the symmetric two-electrode device assembled in 6 M KOH delivered a high energy density of 39.2 Wh kg?1 and excellent chemical stability (90% capacitance retention after 10,000 cycles at 5 A g?1). Such prominent results might provide a new perspective on the value-added application of the renewable biomass resources in the electrochemical field. |
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Keywords: | Biomass Hierarchically porous structure Carbon materials Supercapacitor High energy density |
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