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Applying chemical engineering concepts to non-thermal plasma reactors
Authors:Pedro AFFONSO NOBREGA  Alain GAUNAND  Vandad ROHANI  
Affiliation:1. MINES ParisTech, PSL Research University, PERSEE—Centre for Processes, Renewable Energy and Energy Systems, CS 10207 rue Claude Daunesse F-06904 Sophia Antipolis Cedex, France;2. MINES ParisTech, PSL Research University, CTP-Centre for Thermodynamics of pProcesses, 35 rue St Honoré F-77300 Fontainebleau, France
Abstract:Process scale-up remains a considerable challenge for environmental applications of non-thermal plasmas.Undersanding the impact of reactor hydrodynamics in the performance of the process is a key step to overcome this challenge.In this work,we apply chemical engineering concepts to analyse the impact that different non-thermal plasma reactor configurations and regimes,such as laminar or plug flow,may have on the reactor performance.We do this in the particular context of the removal of pollutants by non-thermal plasmas,for which a simplified model is available.We generalise this model to different reactor configurations and,under certain hypotheses,we show that a reactor in the laminar regime may have a behaviour significantly different from one in the plug flow regime,often assumed in the non-thermal plasma literature.On the other hand,we show that a packed-bed reactor behaves very similarly to one in the plug flow regime.Beyond those results,the reader will find in this work a quick introduction to chemical reaction engineering concepts.
Keywords:non-thermal plasma  chemical engineering  dielectric barrier discharge (DBD)  corona discharge  plug flow reactor  volatile organic compounds  
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