Nanoparticle formation in H2O/N2 and H2O/Ar mixtures under irradiation by 20 MeV protons and positive corona discharge |
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Authors: | Masashi Imanaka Shigeo Tomita Suguru Kanda Mitsuteru Fujieda Kimikazu Sasa Jens Olaf Pepke Pedersen Hiroshi Kudo |
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Affiliation: | 1. RIKEN (The Institute of Physical and Chemical Research), Hirosawa 2-1, Wako, Saitama 351-0198, Japan;2. Institute of Applied Physics, University of Tsukuba, Tennoudai 1-1-1, Tsukuba, Ibaraki 305-8573, Japan;3. Tandem Accelerator Complex, University of Tsukuba, Tennoudai 1-1-1, Tsukuba, Ibaraki 305-8577, Japan;4. National Space Institute, Technical University of Denmark, Juliane Maries Vej 30, 2100 Copenhagen, Denmark |
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Abstract: | To investigate the contribution of ions to gas nucleation, we have performed experiments on the formation of water droplets in H2O/N2 and H2O/Ar gas mixtures by irradiation with a 20 MeV proton beam and by positive corona discharge. The size of the formed nanoparticles was measured using a differential mobility analyzer equipped with a Faraday cup electrometer. Using the proton beam, droplets around 10 nm in diameter were observed for both positively and negatively charged particles, but none were found when the corona discharge was used. This implies the importance of the presence of both positive and negative ions for the formation of nanosize droplets, which attract each other by Coulomb interactions, enhancing the collision frequency and leading to the formation of the 10 nm droplets. |
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