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Photo-Assisted Processes for Improved Catalytic Activity and Selectivity of Environmentally Harmful Emissions
Authors:Ljungström  Sten  Chakarov  Dinko  Bergeld  Johan  Johansson  Stefan  Kasemo  Bengt
Affiliation:(1) Competence Centre for Catalysis and Department for Applied Physics, Chalmers University of Technology and Göteborg University, S-412 96 Göteborg, Sweden
Abstract:Photoenhanced activity of several supported noble metal/metal oxide combinations has been explored. Significant activity is observed for supported Pt and Pd samples. Specifically, the so called light-off temperatures for CO oxidation are found to decrease upon illumination. Evidence for a photocatalytic non-thermal mechanism rather than a photo-assisted thermal process is found through the wavelength dependence for CO oxidation on a Pt/alumina catalyst. The difficulty of separating real photocatalytic from other photo-assisted effects in the case of porous samples is discussed.
Keywords:CO oxidation  photocatalysis  suppported noble metal catalysts  emission cleaning
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