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Selective catalytic reduction of NOx with propene over double wash-coat monolith catalysts
Authors:Chan-Soon Kang   Young-Jae You   Ki-Joong Kim   Tae-hee Kim   Seong-Jun Ahn   Kyong-Hwan Chung   Nam-Cook Park   Shoichi Kimura  Ho-Geun Ahn  
Affiliation:

aDepartment of Chemical Engineering, Sunchon National University, 315 Maegok-dong, Suncheon-si, Jeonnam 540-742, Republic of Korea

bKorea Institute of Culture Technology, Gokseong-kun, Jeonnam 516-853, Republic of Korea

cDepartment of Chemical Engineering, Chonnam National University, 300 Yongbong-dong, Buk-gu, Gwangju 500-757, Republic of Korea

dDepartment of Chemical Engineering, Oregon State University, 102 Gleeson Hall, Corvallis 97331-2702, USA

Abstract:Selective catalytic reduction (SCR) among the approaches for alleviating NOx emission was much attracted. Zeolites have the advantage for adsorption of propene, and noble metal catalyst has the advantage for oxidation of NO to NO2. Pt (or Au)/Al2O3 (or SiO2) were used as the lower layer of double wash-coated monolith catalysts. Zeolites (H-mordenite or ZSM-5) were coated as the upper layer. The catalytic performance of the double wash-coated catalyst was, remarkably, improved. Also, temperature window was shifted to lower temperature and broadened. It was known that the combined noble metal monolith catalyst with zeolite was very effective in removing NOx by SCR with hydrocarbons.
Keywords:NOx   Double wash-coat   Monolith   SCR   Propene
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