Selective catalytic reduction of NO by NH3 on Cu (II) ion-exchanged offretite prepared by different methods |
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Authors: | Arous W. Tounsi H. Djemel S. Ghorbel A. Delahay G. |
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Affiliation: | (1) Département de chimie, FST, Laboratoire de Chimie des Matériaux et Catalyse, Campus Universitaires, 1060 Tunis, Tunisia;(2) Laboratoire de Matériaux Catalytiques et Catalyse en Chimie Organique, UMR 5618 du CNRS, ENSCM, 8 rue de l’école Normale, 34296 Montpellier cedex, France |
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Abstract: | The influence of the preparation method on the NO–SCR by NH3 activity of Cu-OFF catalysts has been studied on presence of oxygen. The catalysts structure and the nature of copper species have been investigated by XRD, 27Al MAS NMR, UV-visible spectroscopy and H2-TPR. Among the examined preparation methods, the ionic exchange in aqueous solution gives the highest efficient catalyst in NO-SCR. It is shown that Cu cationic species are formed in large extent with this method despite the presence of minor amounts of small oxide clusters. |
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Keywords: | SCR NH3 NO Cu-OFF |
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