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Synthesis and Characterization of CNT Composites for Laser‐Generated Ultrasonic Waves
Authors:Patrick Oser  Oliver Düttmann  Fabian Schmid  Levin Schulte‐Spechtel  Christian U Große  Datong Wu
Abstract:In the last few years, extensive progress in ultrasonic wave generation by using multiwalled carbon nanotubes (MWCNTs) in combination with polydimethylsiloxane (PDMS), functional composites, has been achieved. Due to high optical absorption of MWCNTs as perfect absorbers for laser beams and the high thermal expansion coefficient of PDMS, a compact transducer for ultrasonic wave generation at higher frequency can be realized. This study reports a novel method to synthesize MWCNT–PDMS composites deposited on a glass substrate by spray coating, which is done in a short time of 2 h. The layers (0.9–32.2 µm) show low optical transmission properties of 13.9–0.0% at a wavelength of 1047 nm. Apart from using a 1% Triton‐X‐100 stock solution and then diluted to a 0.1% relatively nonhazardous solution, no toxic chemicals are used. The Triton‐X‐100 solution is not hazardous for lab handling and is a commonly used lab detergent for the treatment of biological cells. The achieved sound pressure level is 3.4 MPa with a frequency bandwidth of 9.7 MHz. These results show the potential for a fast and nontoxic production of laser‐generated ultrasonic transducers, which can be used well in the field of nondestructive material testing of layered materials or in medicine with an appropriate frequency range.
Keywords:laser‐generated ultrasonic waves  multi‐walled CNTs  nanocomposites  nanoparticles  photophysics  spray‐coating methods
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