Heterodyne detection of tunable FIR sidebands

Continuously tunable far infrared (FIR) laser sidebands have been generated in a Schottky diode by nonlinear mixing the radiation from an optically pumped FIR laser operating between 0.6 and 3 THz with that from a microwave source in the 2-4 GHz range. A very sensitive heterodyne detection is adapted to detect the sidebands generated not only at the sum or difference frequency of the two radiations, but also, for the first time in the FIR region, those related to the mixing of the FIR radiation with the second and third harmonics of the microwaves. The high selectivity of the superheterodyne detection allows easy separation of the various sidebands. The global tunability of this system is 2 × 10 GHz for the more powerful FIR emission lines. To demonstrate the tunability of the device absorption signals of several molecules are presented in the whole range of operation of the system (0.6-3 THz) using either direct or lock-in detection techniques.