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Near-field spectroscopy of single quantum dots at room temperature
Authors:K Ikeda  K Matsuda  H Saito†  K Nishi†  & T Saiki‡
Affiliation:Kanagawa Academy of Science and Technology, 408 KSP-East, 3-2-1 Sakado, Takatsu-ku, Kawasaki 213-0012, Japan;NEC, 34 Miyukigaoka, Tsukuba 305–8501, Japan;The University of Tokyo, 7–3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, Japan
Abstract:The observation of photoluminescence spectra of self-assembled single InGaAs quantum dots at room temperature was performed under weak excitation conditions using a near-field scanning optical microscope. Operation in illumination-collection mode with a highly sensitive double-tapered optical fibre probe enabled detection of weak photoluminescence signals at room temperature with high efficiency and high spatial resolution. Each single quantum dot was imaged with a spatial resolution of about 250 nm, which corresponded to a quarter of the wavelength of the photoluminescence from quantum dots. The photoluminescence yields of individual quantum dots were widely distributed and were found to decrease with photoluminescence energy. This result serves as a clue to be pursued for better understanding of the thermal excitation of the carrier from confined states in quantum dots.
Keywords:Double-tapered optical fibre probe  emission linewidth  illumination-collection mode  inter-level spacing  near-field scanning optical microscopy  photoluminescence  quantum dot  
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