Transparent perovskite glass-ceramics for visual optical thermometry |
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Authors: | Qihua Yang Lei Zhao Zhaohui Fang Ze Yang Jiangyan Cao Yiyu Cai Dacheng Zhou Xue Yu Jianbei Qiu Xuhui Xu |
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Affiliation: | 1. Faculty of Materials Science and Engineering, Kunming University of Science and Technology, Kunming 650093, China;2. School of Physics and Opto-Electronic Technology, Baoji University of Arts and Sciences, Baoji 721016, China;3. Key Laboratory of Advanced Materials of Yunnan Province, Kunming 650093, China |
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Abstract: | Optical thermometers have aroused considerable attention in recent years,and the increasing demand of sensitivity for practical application encourages the investigation on developing innovative non-contact optical thermo metric materials with higher sensitivity and accuracy.Perovskite quantum dots(QDs)with excellent temperature-dependence optical properties,provide a feasible approach to realizing the detection of temperature change,however,their poor high temperature thermal stability and the facile realization to obtain the production remain a daunting challenge.Herein,growing Tb~(3+)-doped CsPbl_3 QDs in situ in borosilicate glass is proposed,which ensures the phase stability,and high-efficiency florescence output of the all-inorganic perovskite as a temperature sensor.A higher absolute and relative temperature sensitivity(0.0398 K~(-1) and 7.12%/K,respectively),along with the visible color change from orange-red to yellow-green with the increase of temperature is accomplished.Notably,the repeatable florescence intensity of Tb~(3+)-doped CsPbl_3 QDs under high temperature enables their temperature sensing application. |
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Keywords: | Thermometry Thermal stability Visual change Rare earths |
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