Cr4+ lasers: present performance and prospects for newhost lattices

Cr-doped lasers, based on forsterite and YAG, provide broadly tunable power in the 1.25-μm and 1.45-μm regions. Performance data on tuning range, pumping, output power, and thermal management for these lasers is reviewed. Potential new crystals for Cr⁴⁺ should have heavy atoms to reduce lattice phonon frequencies, a distorted tetrahedral cage for the Cr⁴⁺ ion, and possibly an octahedral site for Cr³⁺. Possible materials include monticellite and diopside     

Optimization of Broadband Gain Spectra of Cr $^{hbox{4}+}$:YAG Crystal Fiber Amplifier

In this paper, we present energy level, transition configuration, and numerical model of Cr³⁺/Cr⁴⁺:YAG crystal fiber amplifier for the first time, to the best of our knowledge. The rate and power propagation equations of the numerical model are solved and analyzed. The active ion concentration, length of the doped fiber, and pump power are optimized to maximize the bandwidth of the gain spectra. The effect of temperature on the gain spectra is also discussed. It is shown that based on analysis of the absorption spectra and emission spectra, Cr⁴⁺:YAG crystal is a three-level system, and the broadband gain of Cr ³⁺/Cr ⁴⁺ :YAG crystal fiber is attributed to the broad emission of Cr⁴⁺ ions, especially tetrahedral Cr ⁴⁺ in YAG. When excited at 800 nm, optimal fibers have ultrabroad gain spectra in the range of 1.2-1.65 mum, which cover the low-loss windows of the all-wave fiber without absorption peak caused by OH^- group.     

Highly efficient diode-pumped 3-μm Er3+:BaY2F8 laser

A systematic investigation on a series of monoclinic Er³⁺ :BaY₂F₈ crystals with different dopant concentrations (C_Er=5%-30%) and crystal orientations was conducted to optimize the laser performance in this new 3-μm laser medium by laser diode pumping. The highest slope efficiency of 32% near the quantum defect (35%) was obtained with a 10% doped Er³⁺:BaY₂F₈ crystal with the orientation (010) and a length of 3.5 mm. A maximum output power of 160 mW was achieved at an absorbed pump power of 550 mW at a wavelength of 970 nm     

High-power CW deep-UV coherent light sources around 200 nm based on external resonant sum-frequency mixing

We report pure continuous-wave (CW) high-power (>100 mW) deep-ultraviolet (DUV) light sources emitting around 200-nm spectral region based on singly resonant sum-frequency mixing (SRSFM). Efficient DUV generation is made possible by use of a Brewster-cut CsLiB/sub 6/O/sub 10/ (CLBO) crystal near noncritically phase-matched (NCPM) condition for the SFM of 1-/spl mu/m output of neodymium lasers. The CW radiation of fifth-harmonic wavelength of a neodymium laser at 213 nm was generated by the SFM of enhanced 1064-nm radiation with single-passing 266-nm radiation produced by external-resonant frequency doubling of a 532-nm green laser. With 1.8 W of 266-nm radiation incident upon a CLBO crystal, as much as 180 mW of CW 213-nm power has been produced. The sub-200-nm CW radiation with 140-mW power has also been achieved by SFM of 1064 nm with 244-nm radiation from a frequency-doubled Argon-ion laser in the CLBO crystal operated near the NCPM condition.     

Diode-pumped neodymium lasers repetitively Q-switched by Cr4+:YAG solid-state saturable absorbers

We report on the experimental results of a continuously diode-laser pumped Nd:YAG laser, operating at 1064 nm and repetitively Q-switched by a Cr⁴⁺:YAG solid-state saturable absorber. End-pumping the Nd:YAG with a 10-W fiber-coupled diode-laser we could either optimize the energy or the average output power, depending on the choice of the saturable absorber and the output coupler. The maximum energy was ≈200 μJ in single TEM₀₀, 17 ns pulses at 6 kHz, whereas a maximum average power of ≈2 W with 32-ns pulses at 20 kHz was obtained. We also present preliminary results of a repetitively Q-switched Nd:YVO₄ laser at 1064 nm. The repetitive Q-switching operation is described by an improved model, which accounts for the behavior of both the active medium and the solid-state saturable absorber. The results of the model agree fairly well with the experimental data. Experimental results of second harmonic conversion are also reported and interpreted using a depleted pump model     

High-power VCSELs: single devices and densely packed 2-D-arrays

We report on vertical-cavity surface-emitting lasers (VCSELs) and laser arrays providing high output powers in the 980-nm wavelength regime. Extensive investigations on size scaling behavior of single top- and bottom-emitting devices concerning fundamental electrooptical and thermal properties show limits of attainable output characteristics. Maximum experimentally achieved continuous-wave (CW) optical output powers at room temperature are 180 and 350 mW for top- and bottom-emitting VCSELs, respectively. Detailed analysis on the thermal interaction between closely spaced elements have been carried out to describe the thermally induced power limitations of two-dimensional arrays. Fabricated heat sunk bottom-emitting arrays of 23 elements and 40-μm aperture size of individual elements show output powers of 0.56 W CW at room temperature and 0.8 W actively cooled, resulting in 0.33 kW/cm² and 0.47 kW/cm² maximum spatially averaged optical power density, respectively     

Comparative Performance of Passively Q-Switched Diode-Pumped Yb 3+-Doped Tungstate and Garnet Lasers Using Cr 4+:YAG Saturable Absorber

We investigated the continuous wave (CW) free-running and repetitive modulation in the kilohertz frequency domain of a passively Q-switched diode-pumped Yb:YAG, Yb:GGG, and Yb:KYW lasers by using Cr⁴⁺:YAG as a saturable absorber. The results presented in this paper are focused on the design of a passively Q-switched Yb-doped garnets or Yb-doped tungstates microlasers. The free-running performance of Yb:YAG, Yb:GGG, Yb:KGW, and Yb:KYW were characterized, and experimental parameters such as gain and loss were evaluated. We carried out a fit between our experimental results and an existing numerical model, which relates the experimental and the physical parameters of the ytterbium diode-pumped system to the minimal threshold pumping power. The best performance among the laser crystals was obtained for Yb:YAG laser. A maximum peak power of ap4.5 kW at an average output power of 1.32 W was extracted with an extraction efficiency of ap25%.     

Advanced Ti:Er:LiNbO3 waveguide lasers

This paper reviews the latest developments of diode-pumped Ti,Er:LiNbO₃ waveguide lasers emitting at wavelengths around 1.5 μm. In particular, harmonically mode-locked lasers, Q-switched lasers, distributed Bragg reflector (DBR)-lasers, and self-frequency doubling lasers are discussed in detail. Supermode stabilized mode-locked lasers have been realized using a coupled cavity concept; a side mode suppression ratio of 55 dB has been achieved at 10-GHz pulse repetition rate with almost transform limited pulses. Q-switched lasers with a high extinction ratio (>25 dB) intracavity electrooptic switch emitted pulses with a peak power level up to 2.5 kW and a pulsewidth down to 2.1 ns at 1-kHz repetition frequency. Numerical simulations for both lasers are in a good, almost quantitative agreement with experimental results. A DBR-laser of narrow linewidth (≈3 GHz) with a permanent (fixed) photorefractive grating and 5 mW output power has been realized. Self frequency doubling lasers have been fabricated with a periodic microdomain structure inside an Er-doped laser cavity; simultaneous emission at the fundamental wavelength, 1531 nm, and at the second harmonic wavelength, 765 nm, has been obtained     

Diode-pumped tunable Yb:YAG miniature lasers at room temperature:modeling and experiment

We present a simple design rule for diode-laser pumped quasi-three-level lasers by using the M² factor. The validity of this model was demonstrated by diode-pumped Yb:YAG laser experiments. The maximum output power of 1.33 W and optical slope efficiency of 63% were obtained in a 400-μm Yb:YAG chip miniature laser. Using a 200-μm Yb:YAG chip, a 70% optical slope efficiency was reached. In a coupled-cavity configuration, with a quartz birefringent tuning filter, 8.2 THz (29 nm) of tuning was obtained at room temperature. By changing to a calcite birefringent filter, single-axial-mode oscillation with an output power of 500 mW was observed     

Ce3+:LiCaAlF6 crystal for high-gain orhigh-peak-power amplification of ultraviolet femtosecond pulses and newpotential ultraviolet gain medium: Ce3+:LiSr0.8Ca0.2AlF6

To develop high-peak-power ultrashort pulse laser systems in the ultraviolet region, a large Ce³⁺:LiCaAlF₆ (Ce:LiCAF) crystal, a tunable ultraviolet laser medium with large saturation fluence and broad gain spectrum width, was grown successfully with a diameter of more than 70 mm. To demonstrate high small signal gain, a four-pass confocal amplifier with 60 dB gain and 54 μJ output energy was constructed. Chirped pulse amplification (CPA) in the ultraviolet region was demonstrated using Ce:LiCAF for higher energy extraction. A modified bow-tie-style four-pass amplifier pumped by 100-mJ 266-nm 10-Hz pulses from a Q-switched Nd:YAG laser had 370-times gain and delivered 6-mJ 290-nm pulses. After dispersion compensation, the output pulses can be compressed down to 115 fs. This is the first ultraviolet, all-solid-state high-peak-power CPA laser system using ultraviolet gain media, and this demonstration shows further scalability of the Ce:LiCAF CPA system. Additionally, a new gain medium, Ce³⁺ :LiSr_0.8Ca_0.2AlF₆, with longer fluorescence lifetime and sufficient gain spectrum width over 18 nm was grown to upgrade this system as a candidate for a final power amplifier gain module     

Wavelength-swept fiber laser with frequency shifted feedback andresonantly swept intra-cavity acoustooptic tunable filter

This paper concerns a wavelength-swept fiber laser (WSFL) incorporating frequency shifted feedback and an intracavity passband filter, in which the wavelength of the modeless output is linearly, continuously and repeatedly tuned (in time) over a given range by modulation of the filter peak wavelength and filter strength. We show both numerically and experimentally that amplifier noise plays a key role in determining the operation of frequency-shifted fiber laser systems and that a “noisy” amplifier can be used to suppress the natural tendency of such lasers to pulse, allowing for continuous wave, modeless operation. Furthermore, we show that significant narrowing of a WSFL instantaneous swept linewidth can be obtained if the filter peak transmission wavelength is resonantly swept so as to follow the wavelength shift per pass due to the acoustooptic frequency shift. Using these ideas we go on to demonstrate and characterize a high-power diode-driven Er³⁺/Yb³⁺ WSFL incorporating a bulk-optic acoustooptic tunable filter (AOTF). Linewidths as narrow as 9 GHz, sweep ranges up to 38 nm and output powers as high as 100 mW are obtained. Furthermore, we demonstrate the generation of user definable average spectral output by synchronous modulation of the filter strength and multiwavelength pulsed output at higher sweep rates. Excellent agreement between the experimental results and those of the numerical modeling is obtained. Our simulations show that reduced linewidth (<0.02 nm) and improved scan linearity should be readily achievable with realistic system improvements. We believe such sources to be of considerable physical and practical interest, with applications ranging from sensor array monitoring and device characterization through to low-coherence interferometry     

High-power continuous-wave intracavity frequency-doubled Nd:GdVO/sub 4/-LBO laser under diode pumping into the emitting level

The continuous-wave high power laser emission of Nd:GdVO/sub 4/ at the fundamental wavelength of 1.06 /spl mu/m and its 531-nm second harmonic obtained by intracavity frequency doubling with an LBO nonlinear crystal is investigated under pumping by diode laser at 808 nm (on the /sup 4/I/sub 9/2//spl rarr//sup 4/F/sub 5/2/ transition) and 879 nm (on the /sup 4/I/sub 9/2//spl rarr//sup 4/F/sub 3/2/ transition). It is shown that, in spite of a lower absorption at 879 nm, the infrared emission is comparable under these two wavelengths of pump. The green emission performances were, however, improved by the 879 nm pump: 5.1 W at 531 nm with M/sup 2/=1.46 and 0.31 overall optical-to-optical efficiency was obtained from a 3-mm-thick 1-at.% Nd:GdVO/sub 4/ laser medium and a 10-mm-long LBO nonlinear crystal in a Z-type cavity for 16.5 W pump power. In similar conditions, the maximum green power for the 808 nm pump was 4.4 W, with 0.26 overall optical-to-optical efficiency and M/sup 2/=3.40 beam quality; at this pump wavelength the green emission shows evident saturation for pump power in excess of 9.9 W. This behavior is connected with the enhanced heat generation under 809-nm pumping, as evidenced by the increased thermal lensing of the fundamental emission. A careful alignment of the laser enables emission almost free of chaotic intensity fluctuations.     

Cryogenic Yb3+-Doped Solid-State Lasers

Cryogenically cooled solid-state lasers promise a revolution in power scalability while maintaining a good beam quality because of significant improvements in efficiency and thermo-optic properties. This is particularly true for Yb lasers because of their relatively low quantum defect and relatively broadband absorption even at cryogenic temperatures. Thermo-optic properties of host materials, including thermal conductivity, thermal expansion, and refractive index at low temperature, are reviewed and data presented for YAG (ceramic and single crystal), GGG, GdVO₄, and Y₂O₃. Spectroscopic properties of Yb:YAG and Yb:LiYF₄ (YLF) including absorption cross sections, emission cross sections, and fluorescence lifetimes at cryogenic temperatures are characterized. Recent experiments have pushed the power from an end-pumped cryogenically cooled Yb:YAG laser to 455-W continuous-wave output power from 640-W incident pump power at an of M² 1.4.     

CW solid-state ultraviolet laser for optical disk masteringapplication

We have built a prototype laser head that emits 355-nm ultraviolet light in CW mode. The system is based on nonlinear sum-frequency mixing using a β-BaB₂O₄ (BBO) crystal in an external resonator in which two input emissions at 1064 and 532 nm are resonantly enhanced simultaneously. The output exhibits promising characteristics as the master recording laser source, in terms of beam shape and intensity stability. The result of reliability testing of the system in 1000-h real-time operation is also discussed     

Influence of doping concentration on the power performance of diode-pumped continuous-wave Tm/sup 3+/:YAlO/sub 3/ lasers

We investigated the effect of thulium ion concentration on the continuous-wave (CW) power performance of diode single-end-pumped thulium-doped YAlO/sub 3/ (Tm:YAP) lasers. Three samples with 1.5%, 3%, and 4% Tm/sup 3+/ concentration were examined at 18/spl deg/C. Lifetime and fluorescence measurements were further performed to assess the strength of cross relaxation and nonradiative decay. Our results showed that in single-end-pumped configurations, the best CW power performance was obtained with the 1.5% Tm:YAP sample, and laser performance of the samples degraded monotonically with increasing Tm/sup 3+/ concentration. By using 9.5 W of incident pump power at 797 nm, a maximum of 1430 mW of output power was obtained with the 1.5% Tm:YAP sample and 2% output coupler. We discuss how the effects of cross relaxation, reabsorption, nonradiative decay, and internal heating vary with increasing concentration. Spectroscopic measurements and rate-equation analysis suggest that cross relaxation should already be effective in samples with 1.5% Tm/sup 3+/ ion concentration and doping concentrations larger than 4% will lead to degradation in power performance due to higher nonradiative decay rates and larger reabsorption losses.     

High-power and high-efficiency operation of a CW-diode-side-pumpedNd:YAG rod laser

We have demonstrated high-power and high efficiency performance of a continuous-wave (CW) Nd:YAG laser with a simple and scalable side-pumping configuration. The maximum output power of 147 W was obtained in low brightness operation of M²=45. The corresponding electric efficiency is 14.8%. To our knowledge, this is the highest value reported for diode side-pumped Nd:YAG lasers. By using a rate and photon transport calculation, we have estimated the pumping efficiency of 72%. High brightness operation was also carried out by applying bifocusing compensation of the Nd:YAG rod. The brightness of 272 MW/cm² sr with beam quality of M²=5.9 and output power of 107 W was obtained at the electric efficiency of 11.6%. The brightness and the electric efficiency are comparable with those of industrial high-power CO₂ lasers that have been the first option for industrial applications     

Improved output performance of high-power VCSELs

The intention of this paper is to report on state-of-the-art high-power vertical-cavity surface-emitting laser diodes (VCSELs), single devices as well as two-dimensional (2-D) arrays. Both approaches are studied in terms of electrooptical characteristics, beam performance, and scaling behavior. The maximum continuous wave (CW) output power at room temperature of large-area bottom-emitting devices with active diameters up to 320 μm is as high as 0.89 W, which is to our knowledge the highest value reported for a single device. Measurements under pulsed conditions show more than 10-W optical peak output power. Also, the CW performance of 2-D arrays has been increased from 0.56 W for 23 elements to 1.55 W for 19 elements due to significantly improved heat sinking. The extracted power densities spatially averaged over the area close to the honeycomb-like array arrangement raised from 0.33 kW/cm² to 1.25 kW/cm². Lifetime measurements have proven acceptable reliability for over 10000 h at a degradation rate of less than 1% per 1000 h. The emission wavelength of bottom-emitting devices is restricted to about 900 nm or higher due to fundamental absorption in the GaAs substrate. Windowing of the substrate has been studied to allow for shorter wavelength emission     

Fiber-Laser-Pumped Er:YAG Lasers

Hybrid fiber-laser-pumped solid-state lasers exploit high-power cladding-pumped fiber lasers for direct (in-band) pumping of a crystal-based solid-state laser to reduce heating in the laser crystal, and hence allow scaling to higher power in both continuous-wave (CW) and pulsed modes of operation. In this paper, we briefly review the attractions of the hybrid laser approach for generation of output in the ~ 1.6 mum wavelength regime and consider the main design considerations for efficient operation of hybrid lasers based on Er:YAG in both CW and pulsed modes of operation. Examples of hybrid Er:YAG lasers, pumped by Er,Yb codoped fiber lasers at 1532 nm, with CW output powers up to 60 W at 1645 nm and 31 W at 1617 nm and slope efficiencies of 80% and 47% with respect to incident pump power, respectively, are described. In Q-switched mode of operation, pulse energies up to 30.5 mJ were obtained, limited by coating damage. Finally, the prospects for further increase in output power and improvement in overall performance in CW and Q-switched modes of operation will be discussed.     

Laser-Induced Line Patterning of Nonlinear Optical Crystals in Glass

This paper reports the progress in the patterning of nonlinear optical crystal lines on a glass surface by laser irradiation techniques. Two techniques for the patterning of crystal lines have been developed, i.e., rare-earth atom heat processing and transition metal atom heat processing, in which continuous-wave lasers such as Nd:YAG laser (wavelength: lambda = 1064 nm) are irradiated onto the glasses containing rare-earth ions such as Sm³⁺ and Dy³⁺ or transition metal ions such as Ni²⁺ and Cu²⁺. The patterning of lines consisting of nonlinear optical crystals such as beta-BaB₂O₄, SmxBi_1- xBO₃, (Sr,Ba)Nb₂O₆, and LiNbO₃ has been achieved. It is clarified from the azimuthal dependence of second harmonic intensities and polarized micro-Raman scattering spectra that nonlinear optical crystals in the lines are highly oriented along the laser scanning direction, i.e., the patterning of single-like crystal lines. It is also possible to pattern two-dimensional crystal bending or curved lines by just changing the laser scanning direction, and such bending crystal lines have a potential for optical waveguides.     

Terahertz Sources Based on Intracavity Parametric Down-Conversion in Quasi-Phase-Matched Gallium Arsenide

We have efficiently generated tunable terahertz (THz) radiation using intracavity parametric down-conversion in gallium arsenide (GaAs). We used three types of microstructured GaAs to quasi-phase-match the interaction: optically contacted, orientation-patterned, and diffusion-bonded GaAs. The GaAs was placed in an optical parametric oscillator (OPO) cavity, and the THz wave was generated by difference-frequency mixing between the OPO signal and idler waves. The OPO used type-II phase-matched periodically poled lithium niobate as a gain medium and was synchronously pumped by a mode-locked laser at 1064 nm (7 ps and 200 nJ at 50 MHz). With center frequencies spanning 0.4-3.5 THz, 250-GHz bandwidth radiation was generated. We measured two orders of optical cascading generated by the mixing of optical and THz waves. In a doubly resonant oscillator (DRO) configuration, the efficiency increased by 21times over the singly resonant oscillator performance with an optical-to-THz efficiency of 10^-4 and average THz power of 1 mW. The GaAs stabilized the DRO by a thermooptic feedback mechanism that created a quasi- continuous-wave train of THz pulses.