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《Materials Letters》2006,60(25-26):3088-3090
In this paper, we doped p-type conductivity dehydrated nanotubed titanic acid (DNTA) into insulator polymer poly(methyl methacrylate) (PMMA). The electric properties of this nanocomposite were investigated. The photoluminescence efficiency of fluorescent dye 4-(dicyanomethylene)-2-t-butyl-6(1,1,7,7-tetramethyljulolidyl-9-enyl)-4H-pyran (DCJTB) in PMMA matrix was enhanced by doping with DNTA. Moreover, screen effect by DNTA with high permittivity caused the emission from DCJTB to be blue-shifted. 相似文献
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Ab initio method was employed to determine the mechanism of alkylation reaction of 2-butene with isobutane. The results indicated that 2-butene is rapidly protonated to form sec-butyl carbonium ion, which then reacts with isobutane to form tert-butyl carbonium ion. The resulting carbonium ion is then deprotonated to form isobutene that reacts rapidly with tert-butyl carbonium ion to form trimethylpentane (TMP) carbonium ion. Finally, the TMP+ carbonium ion is converted to TMP via the hydride transfer process. The transition states of the interactions were obtained by using the SCAN method (a calculation key word for potential energy surface) first and then the intrinsic reaction coordinates were traced using the Gaussian program. In addition, the energy changes and geometric parameters of the interactions were analyzed. The computed results indicated that the energy barriers are close to or less than zero for the interaction of isobutane with protonated 2-butene or for the interaction of tert-butyl carbonium ion with isobutene, suggesting rapid reaction steps of the carbonium ions. The 2,2,3-TMP is kinetically controlled, while the formation of 2,2,4-TMP is controlled by reaction equilibrium. The calculated results were in good agreement with the experimental results. 相似文献
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Bian Jia-Wang Zhan Huangying Wang Naiyan Li Zhichao Zhang Le Shen Chunhua Cheng Ming-Ming Reid Ian 《International Journal of Computer Vision》2021,129(9):2548-2564
International Journal of Computer Vision - We propose a monocular depth estimation method SC-Depth, which requires only unlabelled videos for training and enables the scale-consistent... 相似文献
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Gu Min Gu Yanhui Luo Weilan Xu Guandong Yang Zhenglu Zhou Junsheng Qu Weiguang 《Neural computing & applications》2021,33(11):6009-6025
Neural Computing and Applications - Semantic understanding is an essential research issue for many applications, such as social network analysis, collective intelligence and content computing,... 相似文献
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The spectra of the optical absorption coefficient in low absorption region are obtained by using a normalization procedure
for the photoconductivity spectra. The results are explained in terms of the optical transition of electrons from localized
states in the exponential valence band tail and in dangling bond states 1.0 eV below the conduction band edge to extended
conduction band states. Then the density of the gap states below the Fermi levelE
F
is obtained. From the investigation of recombination kinetics, the average density of the gap states over the range of
) and the density of the gap states above the Fermi levelE
F
are obtained. These indicate that the width of the conduction band tail is smaller than that of the valence band tail. 相似文献