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排序方式: 共有3866条查询结果,搜索用时 15 毫秒
1.
《International Journal of Hydrogen Energy》2022,47(28):13604-13615
In this study, seven mutants from E. aerogenes IAM1183 wildtype were constructed via different strategies including deletion of lactate dehydrogenase, disruption of NADH dehydrogenase gene nuoE, overexpression of pncB and a combination of both to regulate of the NADH supply to enhance hydrogen production. Compared with the parental strain, the hydrogen yields of the strains IAM1183-E, IAM1183-L and IAM1183-EL increased by 23.3, 81.7 and 97.9%, respectively. When the pncB gene was overexpressed, the hydrogen yield of IAM1183/P, IAM1183-E/P, IAM1183-L/P and IAM1183-EL/P increased by 39.0, 6.5, 5.9, and 5.1% compared with the respective original knockout strains. Among them, the total hydrogen yield of strain IAM1183-EL/P with highest production efficiency was 58% higher than IAM1183. Further metabolite analysis indicated that the knockout of nuoE and ldhA, combined with the overexpression of pncB, resulted in a redistribution of the metabolic fluxes in E. aerogenes, which led to an improvement of the hydrogen yield. 相似文献
2.
Effects of ferrite materials as supports (CoFe2O4, NiFe2O4, and Fe3O4) on nano-TiO2 were elucidated by their use in the oxidation of methylene blue. These photocatalysts, which were synthesized by co-precipitation, were characterized by XRD, SEM, EDS and VSM. The crystalline phase of TiO2 onto magnetic MFe2O4 was formed by anatase and rutile. TiO2/CoFe2O4 exhibited the strongest magnetic property of the prepared catalysts, and the photocatalytic efficiencies followed the order TiO2/CoFe2O4 > TiO2/NiFe2O4 > TiO2/Fe3O4. MB decolorization was enhanced with the amount of TiO2 on the photocatalyst, and was moderately affected by the extent of structural distortion of ferrite supports. 相似文献
3.
Shensong Wang Zheng Wu Jie Chen Jiangping Ma Jingshi Ying Shouchen Cui Shigang Yu Yongming Hu Jinhe Zhao Yanmin Jia 《Ceramics International》2019,45(9):11703-11708
In this work, the hydrothermally-synthesized sodium niobate nanowires were used to decompose Rhodamine B dye solution through the piezo-catalytic effect. With the sodium niobate catalyst, a high piezo-catalytic degradation ratio of ~80% was achieved under the excitation of vibration for the Rhodamine B dye solution (~5?mg/l). These active species in the catalytic process, hydroxyl radicals and superoxide radicals with the strong oxidation ability, were also observed, which confirmed the key role of piezoelectric effect for piezo-catalysis. The piezo-catalysis of sodium niobate nanowires provides a high-efficiency and reusable tool in application in depredating the dye wastewater. 相似文献
4.
Crowdsourcing technology offers exciting possibilities for local governments. Specifically, citizens are increasingly taking part in reporting and discussing issues related to their neighborhood and problems they encounter on a daily basis, such as overflowing trash-bins, broken footpaths and lifts, illegal graffiti, and potholes. Pervasive citizen participation enables local governments to respond more efficiently to these urban issues. This interaction between citizens and municipalities is largely promoted by civic engagement platforms, such as See-Click-Fix, FixMyStreet, CitySourced, and OpenIDEO, which allow citizens to report urban issues by entering free text describing what needs to be done, fixed or changed. In order to develop appropriate action plans and priorities, government officials need to figure out how urgent are the reported issues. In this paper we propose to estimate the urgency of urban issues by mining different emotions that are implicit in the text describing the issue. More specifically, a reported issue is first categorized according to the emotions expressed in it, and then the corresponding emotion scores are combined in order to produce a final urgency level for the reported issue. Our experiments use the SeeClickFix hackathon data and diverse emotion classification algorithms. They indicate that (i) emotions can be categorized efficiently with supervised learning algorithms, and (ii) the use of citizen emotions leads to accurate urgency estimates. Further, using additional features such as the type of issue or its author leads to no further accuracy gains. 相似文献
5.
Qiang Xia Tao Feng Xiaowei Lou Ying Wang Yangying Sun Daodong Pan Jinxuan Cao 《International Journal of Food Science & Technology》2020,55(2):669-680
As a decisive attribute, flavour could be influenced by HP treatments through multiple physical and chemical pathways within the high pressure (HP)-assisted meat curing process. This investigation aimed to identify the major pathway influencing volatile flavour patterns of two representative vinasse-cured duck (VCD) products with HP treatments (150–300 MPa/15 min), including wet and dry types, by employing headspace fingerprinting as an untargeted approach. Results suggested that HP treatments greatly lowered moisture contents and increased Warner-Bratzler shear force and thiobarbituric acid reactive substances of the cured samples. According to multivariate models, the volatile flavour patterns of the HP-processed VCD could be clearly separated from the unprocessed samples, but the VCD pressurised at different intensities represented similar volatile fingerprinting, which was validated by e-nose analysis. The discriminant analysis (OPLS-DA) model outlined vinasse-derived ethanol, acetic acid, 3-methyl-1-butanol, 2-methyl-1-butanol, phenethyl alcohol and 2-methyl-3-octanone as the major discriminant aromas across the unpressurised and pressurised samples. 相似文献
6.
《Computers & Mathematics with Applications》2006,51(6-7):1047-1056
Based on the Euler-Maclaurin formula in the spirit of [1], we provide a unified approach to some inequalities of Ostrowski-Grüss type, which include some existing results as special cases. Some illustrative examples are also included. 相似文献
7.
8.
PCC载体氧化剂的制备及应用研究 总被引:3,自引:0,他引:3
制备得到各种有代表性的氯铬酸吡啶(PCC)无机载体氧化试剂,以苯甲醇选择性氧化成苯甲醛为探针反应,考察了载体、反应条件对氧化反应效率的影响,控制各载体氧化剂中PCC的负载量均为1.8 mmol/g。室温下反应,搅拌时间为30 m in,苯甲醇的氧化反应产率为:分子筛65.8%,活性炭75.4%,氧化铝94.6%,硅胶96.9%,相同条件下PCC的产率为65.8%。硅胶是制备负载PCC的优良载体,在载体氧化剂对苯甲醇的氧化反应中,一定范围内增加反应时间和载体加入量都可以提高氧化产率。 相似文献
9.
《Journal of power sources》2006,153(2):413-418
Three types of electrically conducting polymers (ECPs), i.e. polyaniline (PANI), polypyrrole (PPy) and poly-(3,4-ethylenedioxythiophene) (PEDOT) have been tested as supercapacitor electrode materials in the form of composites with multiwalled carbon nanotubes (CNTs). The energy storage in such a type of composite combines an electrostatic attraction as well as quick faradaic processes called pseudo-capacitance. It has been shown that carbon nanotubes play the role of a perfect backbone for a homogenous distribution of ECP in the composite. It is well known that pure conducting polymers are mechanically weak, hence, the carbon nanotubes preserve the ECP active material from mechanical changes (shrinkage and breaking) during long cycling. Apart of excellent conducting and mechanical properties, the presence of nanotubes improves also the charge transfer that enables a high charge/discharge rate. For an optimal use of ECPs in electrochemical capacitors, a special electrode composition with ca. 20 wt.% of CNTs and a careful selection of the potential range is necessary. The capacitance values ranging from 100 to 330 F g−1 could be reached for different asymmetric configurations with a capacitor voltage from 0.6 to 1.8 V. It is also noteworthy that such a type of ECP/CNTs composite does not need any binding substance that is an important practical advantage. 相似文献
10.
《Energy Policy》2005,33(14):1807-1823
Project-based mechanisms for emissions reductions credits, like the Clean Development Mechanism, pose important challenges for policy design because of several inherent characteristics. Participation is voluntary, so it will not occur without sufficient credits. Evaluating reductions requires assigning an emissions baseline for a counterfactual that cannot be measured. Some investments have both economic and environmental benefits and might occur anyway. Uncertainty surrounds both emissions and investment returns, and parties to the project are likely to have more information than the certifying authority. The certifying agent is limited in its ability to design a contract that would reveal investment intentions. As a result, rules for benchmarking emissions may be systematically biased to overallocate, and they also risk creating inefficient investment incentives. This paper evaluates, in a situation with asymmetric information, the efficacy of the main baseline rules currently under consideration: historical emissions, an average industry emissions standard, and expected emissions. 相似文献