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排序方式: 共有91条查询结果,搜索用时 78 毫秒
1.
Defect‐Rich Ultrathin ZnAl‐Layered Double Hydroxide Nanosheets for Efficient Photoreduction of CO2 to CO with Water 下载免费PDF全文
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Kate Sanders Sally Fincher Dennis Bouvier Gary Lewandowski Briana Morrison Laurie Murphy Marian Petre Brad Richards Josh Tenenberg Lynda Thomas Richard Anderson Ruth Anderson Sue Fitzgerald Alicia Gutschow Susan Haller Raymond Lister Renée McCauley John McTaggart Christine Prasad Terry Scott Dermot Shinners-Kennedy Suzanne Westbrook Carol Zander 《Expert Systems》2005,22(3):121-128
Abstract: This paper presents a case study of the use of a repeated single‐criterion card sort with an unusually large, diverse participant group. The study, whose goal was to elicit novice programmers' knowledge of programming concepts, involved over 20 researchers from four continents and 276 participants drawn from 20 different institutions. In this paper we present the design of the study and the unexpected result that there were few discernible systematic differences in the population. The study was one of the activities of the National Science Foundation funded Bootstrapping Research in Computer Science Education project (2003). 相似文献
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A novel and efficient method to produce water dispersible superparamagnetic Fe3O4 nanoparticles is described. Nanoparticles prepared by non‐hydrolytic organic phase methods are subsequently functionalized with (3‐glycidyloxypropyl)trimethoxysilane, a linker that prevents aggregation and is available for subsequent coupling reactions with a wide range of polymers and biomolecules. Ring opening coupling reactions were used to coat the epoxy‐functionalized magnetite nanoparticles with aminated polymers (polyetheramines) or small molecules (arginine). The resulting nanoparticles, with hydrodynamic size of 13 nm, are found to be very stable over extended periods in water or PBS due to the presence of a dense stabilizer layer covalently anchored to the surface. Exceptionally high spin‐lattice relaxivity, r1, values of 17 s?1 mM?1, and low r2/r1 ratios of 3.3–3.8 were exhibited in the clinical MRI frequency range, irrespective of the molecule selected for nanoparticle stabilization. As a result the dispersions are excellent candidates for incorporation into multi‐functional assemblies or for use as positive contrast agent for MRI. 相似文献
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Molecular‐Scale Hybridization of Clay Monolayers and Conducting Polymer for Thin‐Film Supercapacitors 下载免费PDF全文
Jingwen Zhao Simin Xu Kristina Tschulik Richard G. Compton Min Wei Dermot O'Hare David G. Evans Xue Duan 《Advanced functional materials》2015,25(18):2745-2753
Development of electrode materials with well‐defined architectures is a fruitful and profitable approach for achieving highly‐efficient energy storage systems. A molecular‐scale hybrid system is presented based on the self‐assembly of CoNi‐layered double hydroxide (CoNi‐LDH) monolayers and the conducting polymer (poly(3,4‐ethylene dioxythiophene):poly(styrene sulfonate), denoted as PEDOT:PSS) into an alternating‐layer superlattice. Owing to the homogeneous interface and intimate interaction, the resulting CoNi‐LDH/PEDOT:PSS hybrid materials possess a simultaneous enhancement in ion and charge‐carrier transport and exhibit improved capacitive properties with a high specific capacitance (960 F g–1 at 2 A g–1) and excellent rate capability (83.7% retention at 30 A g–1). In addition, an in‐plane supercapacitor device with an interdigital design is fabricated based on a CoNi‐LDH/PEDOT:PSS thin film, delivering a significantly enhanced energy and power output (an energy density of 46.1 Wh kg–1 at 11.9 kW kg–1). Its application in miniaturized devices is further demonstrated by successfully driving a photodetector. These characteristics demonstrate that the molecular‐scale assembly of LDH monolayers and the conducting polymer is promising for energy storage and conversion applications in miniaturized electronics. 相似文献
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Bowden L Faulkner R Clancy C Gallagher A Devine M Gorman D O'Reilly G Dowling A 《Radiation protection dosimetry》2011,147(1-2):210-214
Current guidelines quote tolerances for automatic exposure control (AEC) device performance for X-ray systems as 'Baseline ± X %'. However, in the situation where a baseline figure has not yet been achieved, as in the case of commissioning assessments, this tolerance is not relevant. The purpose of this work is to provide mean doses for direct digital radiography (DDR) X-ray system, operating in AEC, against which comparisons can be made. Dose measurements have been recorded under AEC operation on 29 DDR detectors from three different manufacturers. Two different testing protocols were examined: (1) water equivalent phantoms in front of the DDR detector and (2) aluminium block at the tube head. The average patient exit dose, using the aluminium block was 4.6 μGy with the antiscatter grid in place and 4.0 μGy with the grid removed. Using the water phantoms, the average dose was measured at 17.1 μGy with the antiscatter grid in place and 5.4 μGy with grid removed. Based on these results, it is clear that different testing configurations significantly impact on the measured dose. 相似文献
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Mc Cormack B Geraghty D O'Mahony M 《IEEE transactions on ultrasonics, ferroelectrics, and frequency control》2011,58(11):2461-2468
SAW devices may be configured as strain sensors, providing passive, wireless strain measurement in demanding conditions. A key consideration is the modeling of the sensors, enabling different device designs to be considered. This paper presents a simulation scheme using coupling-of-modes (COM) analysis which allows both the frequency response of a SAW strain sensor and its bias sensitivity to be evaluated. Example applications are presented to demonstrate the use of the model. 相似文献