首页 | 本学科首页   官方微博 | 高级检索  
文章检索
  按 检索   检索词:      
出版年份:   被引次数:   他引次数: 提示:输入*表示无穷大
  收费全文   4784篇
  免费   417篇
  国内免费   52篇
电工技术   115篇
综合类   19篇
化学工业   1334篇
金属工艺   128篇
机械仪表   177篇
建筑科学   211篇
矿业工程   10篇
能源动力   303篇
轻工业   357篇
水利工程   85篇
石油天然气   67篇
武器工业   5篇
无线电   434篇
一般工业技术   769篇
冶金工业   249篇
原子能技术   36篇
自动化技术   954篇
  2024年   3篇
  2023年   88篇
  2022年   136篇
  2021年   305篇
  2020年   268篇
  2019年   330篇
  2018年   381篇
  2017年   356篇
  2016年   326篇
  2015年   212篇
  2014年   358篇
  2013年   523篇
  2012年   356篇
  2011年   409篇
  2010年   242篇
  2009年   236篇
  2008年   145篇
  2007年   87篇
  2006年   100篇
  2005年   60篇
  2004年   37篇
  2003年   41篇
  2002年   36篇
  2001年   22篇
  2000年   18篇
  1999年   12篇
  1998年   22篇
  1997年   13篇
  1996年   19篇
  1995年   13篇
  1994年   7篇
  1993年   12篇
  1991年   8篇
  1990年   9篇
  1987年   5篇
  1986年   4篇
  1985年   5篇
  1984年   7篇
  1983年   7篇
  1982年   6篇
  1981年   3篇
  1980年   2篇
  1979年   2篇
  1978年   4篇
  1977年   5篇
  1976年   2篇
  1975年   7篇
  1970年   1篇
  1969年   1篇
  1965年   1篇
排序方式: 共有5253条查询结果,搜索用时 31 毫秒
1.
2.
Multimedia Tools and Applications - With the rapid development of detecting violent behaviors in surveillance cameras, requests on systems that automatically recognize violent events are expanded....  相似文献   
3.
4.
In this work, we designed a magnetically-separable Fe3O4-rGO-ZnO ternary catalyst, ZnO anchored on the surface of reduced graphene oxide (rGO)-wrapped Fe3O4 magnetic nanoparticles, where rGO, as an effective interlayer, can enhance the synergistic effect between ZnO and Fe3O4. The effects of three operational parameters, namely irradiation time, hydrogen peroxide dosage, and the catalyst dosage, on the photo-Fenton degradation of methylene blue and methyl orange were investigated. The results showed that the Fe3O4-rGO-ZnO had great potential for the destruction of organic compounds from wastewater using the Fenton chemical oxidation method at neutral pH. Repeatability of the photocatalytic activity after 5 cycles showed only a tiny drop in the catalytic efficiency.  相似文献   
5.
In both developing and industrialized/developed countries, various hazardous/toxic environmental pollutants are entering water bodies from organic and inorganic compounds (heavy metals and specifically dyes). The global population is growing whereas the accessibility of clean, potable and safe drinking water is decreasing, leading to world deterioration in human health and limitation of agricultural and/or economic development. Treatment of water/wastewater (mainly industrial water) via catalytic reduction/degradation of environmental pollutants is extremely critical and is a major concern/issue for public health. Light and/or laser ablation induced photocatalytic processes have attracted much attention during recent years for water treatment due to their good (photo)catalytic efficiencies in the reduction/degradation of organic/inorganic pollutants. Pulsed laser ablation (PLA) is a rather novel catalyst fabrication approach for the generation of nanostructures with special morphologies (nanoparticles (NPs), nanocrystals, nanocomposites, nanowires, etc.) and different compositions (metals, alloys, oxides, core-shell, etc.). Laser ablation in liquid (LAL) is generally considered a quickly growing approach for the synthesis and modification of nanomaterials for practical applications in diverse fields. LAL-synthesized nanomaterials have been identified as attractive nanocatalysts or valuable photocatalysts in (photo)catalytic reduction/degradation reactions. In this review, the laser ablation/irradiation strategies based on LAL are systematically described and the applications of LAL synthesized metal/metal oxide nanocatalysts with highly controlled nanostructures in the degradation/reduction of organic/inorganic water pollutants are highlighted along with their degradation/reduction mechanisms.  相似文献   
6.
This study aimed to prepare cisplatin-loaded PEGylated liposomal nanoparticles targeted with folic acid and evaluate their efficacy on liver cancer cell line PLC/PRF/5 (Alexander hepatoma cell line). Nanoparticles were prepared by reverse phase evaporation technique and characterized by dynamic light scattering, scanning electron microscopy, transmission electron microscopy, inductively coupled plasma optical emission spectrometry, Fourier transform infrared spectroscopy, and 3-(4,5-dimethylthiazol-2-yl)-2,5-diphenyltetrazolium bromide techniques. Nanoscale particles with appropriate drug encapsulation efficiency (13%) were prepared. Cytotoxicity results indicated that the superior potency of targeted cisplatin-loaded nanoparticles compared to the nontargeted counterpart with 23% more cytotoxicity. Findings of this study confirmed the potency of targeted PEGylated liposomal nanoparticles.  相似文献   
7.
Wireless Personal Communications - The integration of the Internet of Things (IoT) and cloud environment has led to the creation of Cloud of Things, which has given rise to new challenges in IoT...  相似文献   
8.
To circumvent restrictions of conventional drilling methods, such as slow control actions and inability to drill depleted reservoirs, a drilling method called managed pressure drilling (MPD) has been developed. In MPD, single-phase flow processes can be modeled as a feedback interconnection of a high-order linear system and a low-order nonlinear system. These nonlinearities appear locally both inside and at the boundaries of the computational domain. To obtain a fast simulation platform for real-time purposes (eg, online model-based controller implementation), model order reduction is required for MPD. However, the local nonlinearities render applying model order reduction techniques challenging. In this study, a new approach is proposed to deal with such nonlinearities within the reduced basis (RB) context and it is successfully tested on a model for MPD. Contrary to the classical RB technique, the proposed approach not only does not generate nonphysical spikes at the locations of these local nonlinearities but also yields high speedup factors. The obtained reduced-order model can be used for efficient online simulation and controller design for drilling systems with MPD.  相似文献   
9.
In this study, combustion synthesis of cerium oxide nanoparticles was reported using cerium nitrate hexahydrate as starting material as well as urea, glycine, glucose, and citric acid as fuels. The influence of fuel type on structure, microstructure, band gap, and corrosion inhibition was investigated. X-ray diffraction (XRD) patterns and scanning electron microscopy micrographs showed that CeO2 nanoparticles with different morphologies were obtained depending on the fuel type. Microstructural changes from unreacted gel to sponge-like morphologies were resulted by varying the fuel type from urea, glycine, and glucose to citric acid. In addition to Ce–O bonds, Fourier transform infrared analysis showed carbon bonds of carbonaceous compositions from incomplete combustion which were declined during combustion reaction. Furthermore, corrosion analyses showed that samples synthesized using urea fuel released the most Ce+4 ions and could have better protection than other samples.  相似文献   
10.
Fuel cell-grade hydrogen production has been studied via steam reforming of methanol (SRM) over a series of CuO/ZnO/Al2O3 nanocatalysts fabricated by the combustion method. The effect of sonication and urea/nitrate ratio on the characteristics and catalytic properties of the prepared catalysts has been investigated. The synthesized catalysts were characterized by x-ray diffraction (XRD), field emission scanning electron microscope (FESEM), Particle Size Distribution (PSD), energy dispersive x-ray (EDX), Brunauer-Emmett-Teller (BET) and FTIR analyses XRD patterns showed positive influence of urea/nitrate ratio on CuO and ZnO crystallite sizes. The ultrasonic mixing of primary gel compared with conventional mixing led to lower crystallite size. FESEM images showed that the sample mixed by sonication with a urea/nitrate ratio of 1 had more homogeneous morphology with narrow particle size distribution. EDX results proved the presence of all metals on the surface of the nanocatalysts and better consistence between the gel and surface composition of elements in samples prepared by sonication. Catalytic performance showed that sonication during the mixing of primary gel dramatically increased the methanol conversion. It was also proved that increasing the amount of urea led to lower catalytic activity. The ultrasound-treated nanocatalyst with urea/nitrate?=?1 was the best sample in terms of activity and selectivity. It was stable in the SRM for 1200?min without considerable change in methanol conversion and product selectivity.  相似文献   
设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司  京ICP备09084417号