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1.
Ningbo Gao Kailun Chen Cui Quan Shixi Wu 《International Journal of Hydrogen Energy》2021,46(40):20882-20892
A novel catalyst, Nickel supported over MCM-41 coated ceramic membrane (NMC), was developed using coating method and deposition-precipitation method and applied for steam reforming of real tar in fixed bed. The effects of reaction conditions such as Ni loading amount, reaction temperature and mass ratio of steam to tar were also studied. The good dispersion of Ni nanoparticles and the strong interaction between Ni particles and the support were identified by BET, XRD, H2-TPR and SEM/EDS, resulting in the excellent performance of NMC catalysts. Maximum tar conversion of 96.4% and H2 yield of 98.7 mmol g?1 were obtained using 20NMC with a mass ratio of steam to coal tar of 2 at 800 °C. Moreover, 20 NMC exhibited a good stability in 10 h of lifetime test and the resistance of graphitic carbon formation prone to easier regeneration of catalysts illustrated by Raman spectroscopy. It indicates that the utilization of NMC catalysts for tar steam reforming is a promising way. 相似文献
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We fabricated Sr and Ca-doped CuAlO2 compacts from the mixed powder of CuO, Cu2O, Al2O3, and SrO or CaO by multi-pass hot pressing followed by spark plasma sintering (SPS). The XRD results showed the reaction of CuO, Cu2O and Al2O3 was rather complete and only CuAlO2 single phase was formed when the additive amount of SrO or CaO was appropriate. Multi-pass hot pressing increased the relative density and the usage of plate-like Al2O3 as reaction raw material enhanced the orientation degree. In spite of performance improvement conflicts through elemental doping, density increase and orientation improvement, the measurement on the thermoelectric performance indicated that the electrical resistivity, Seebeck coefficient, power factor, dimensionless figure of merit (ZT) were improved to varying degrees through the synergetic action of elemental doping, density increase, and orientation control. The highest power factor and ZT of the Ca-doped CuAlO2 compacts reached 1.54?×?10?4 W?m?1 K?2 and 0.015 at 973?K, respectively. The thermoelectric performance was higher than those of CuAlO2 at the same temperature in published work before. 相似文献
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利用空间相关性的超短期风速预测 总被引:2,自引:0,他引:2
风速的空间相关性有助于提高其预测质量,特别是在风速突变的情况下。将"离线分类建模,在线匹配模型"的预测思路应用到利用空间相关性的超短期风速预测之中:通过历史数据的时序分析,识别其中各风电场风速存在空间相关性的时段;按其时序特征及其他的条件特征,将观察时窗内的风速序列划分为不同演化形态的样本子集;在离线环境下,分别根据各类形态的训练样本子集优化其专用的预测模型及参数;在线应用时,则根据当下窗口内风速序列的演化形态及相关的条件特征,按匹配所得模型及参数,根据参考风电场的实测数据预测目标风电场的风速。以实际的历史数据验证了所述方法的有效性。 相似文献
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针对基于TOF深度相机的空间目标表面重建的点云源数据容易受到仪器本身、扫描环境、外界干扰等影响,而含有大量的无效点和噪声点,增加了计算负担且影响了重建质量等问题,提出了一种基于随机采样一致性背景分割的点云K 近邻去噪方法,以消除目标数据的异常值和无效点。首先,改进RANSAC算法,通过设置不同的阙值对原始点云进行背景分割,以确保准确提取待重建目标的主要特征。然后,通过K 近邻点云平均算法和双边滤波算法移除离群点,最后使用体素化网格方法实现点云大数据的下采样,简化了目标点云,保留了局部特征,加快了曲面重建速度。实验结果表明,该算法能够有效的剔除噪声点,准确率高,实时性好,满足应用的要求。 相似文献
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介绍简谐振子的工作原理。利用ANSYS软件,采用有限元法创建了简谐振子质量块的实体模型,选择单晶硅作为简谐振子中质量块的材料;设置了模型的材料属性,采用智能分网的方式对模型划分网格,并对质量块模型施加沿x轴水平方向载荷,进行三维的静力分析和模态分析。静力分析得到实体模型的总位移是0.236×10-19μm;模态分析时只对前四阶模型进行了分析,根据其振型图及其总位移的应力云图,得到实体模型的二十阶振动模态的频率是78 001Hz,二十阶的总位移是0.122×10-6μm。 相似文献
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为了缩短惯性约束聚变(ICF)激光装置在靶场区光束引导的总时间为基于光束引导传感器固定子区划分的光束引导方法,提供了引导路径的一种优化方法。通过优化预备子区中心到目标子区中心的角度,最小化对引导总时间有贡献的投射镜的角位移量的总和。以终端光学组件的一种布置为研究对象,以引导目标点为靶室中心的情况为例,介绍了引导路径的优化过程。引导总时间的估计表明,与普通的串行光束引导方法相比,该方法可以很大程度上缩短光束引导的总时间。当预备子区中心与目标子区中心之间的距离为1 mm时,引导总时间可以缩短为采用普通串行引导方法时的0.518倍。 相似文献
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Polyaniline (PANI) nanofibers were successfully synthesized by a modified rapid mixing method, that is, by the rapid mixing of solutions of aniline and ammonium peroxydisulfate in either hydrochloric acid or filtrates of oxidative polymerization of aniline. Scanning electron microscopy examination showed that nanofibrous PANI products were achieved in all cases; this indicated that the initially presented excessive anions and cations had no evident effect on the formation of nanosized PANI. The nanofibrous PANI exhibited excellent dispersability in both water and organic solvents, and an ultraviolet–visible spectrum was successfully recorded by dispersion in cyclohexanone. Composite coatings were fabricated with the dispersions of nanofibrous PANI and solutions of epoxy. Greatly enhanced corrosion protection performances were demonstrated by the coatings loaded with a small quantity of nanofibrous PANI. © 2012 Wiley Periodicals, Inc. J Appl Polym Sci, 2012 相似文献