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1.
The coupling of reaction and diffusion between neighboring active sites in the catalyst pore leads to the spatiotemporal fluctuation in component concentration, which is very important to catalyst performance and hence its optimal design. Molecular dynamics simulation with hard-sphere and pseudo-particle modeling has previously revealed the non-stochastic concentration fluctuation of the reactant/product near isolated active site due to such coupling, using a simple model reaction of A → B in 2D pores. The topic is further developed in this work by studying the concentration fluctuation due to such coupling between neighboring active sites in 3D pores. Two 3D pore models containing an isolated active site and two adjacent active sites were constructed, respectively. For the isolated site, the concentration fluctuation intensifies for larger pores, but the product yield decreases, and for a given pore size, the product yield reaches a peak at a certain reactant concentration. For two neighboring sites, their distance (d) is found to have little effect on the reaction, but significant to the diffusion. For the same reaction competing at both sites, larger d leads to more efficient diffusion and better overall performance. However, for sequential reactions at the two sites, higher overall performance presents at a smaller d. The results should be helpful to the catalyst design and reaction control in the relevant processes. 相似文献
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Yuping Ji Kaixin Song Shiyu Zhang Zhilun Lu Ge Wang Linhao Li Di Zhou Dawei Wang Ian M. Reaney 《Journal of the European Ceramic Society》2021,41(1):424-429
Dense (1-x)wt%CaSnSiO5-xwt%K2MoO4 (CSSO-KMO) composite ceramics were fabricated by the cold sintering process at 180 °C under 400 MPa for 60 min. X-ray diffraction, Energy dispersive X-ray and Raman spectroscopy confirmed that CSSO and KMO coexisted without intermediate phases. As KMO weight fraction increased, relative permittivity (εr) and temperature coefficient of resonant frequency (τf) decreased and the microwave quality factor (Q×f, where f is resonant frequency) increased. Near-zero τf (-0.5 ppm/°C) was obtained for 65 wt%CSSO-35 wt%KMO with εr ~ 9.2 and Q×f ~ 6240 GHz. No chemical reaction between ceramic composites and silver was observed, demonstrating potential for cofiring with Ag-paste. A prototype antenna was fabricated from 65 wt%CSSO-35 wt%KMO composite ceramic with a bandwidth of 144 MHz @ -10 dB, a gain of 5.7 dBi and a total efficiency of 88.4 % at 5.2 GHz, suitable for 5 G mobile communication systems. 相似文献
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This study compared the effects of 4K organic light‐emitting diode (OLED) and liquid‐crystal display (LCD) TVs on human visual task performance and fatigue when viewing moving pictures. In experiments conducted, subjects were asked to locate 35 icons among a total of 276 on‐screen icons at four moving picture speeds. From the results obtained, it was determined that OLED TVs (emissive type) exhibit superior characteristics for hit rate and false alarm rate compared with LCD TVs (non‐emissive‐type). The evaluation results of a simulator sickness questionnaire administered to ascertain fatigue levels also indicated that OLED TVs induce relatively little fatigue at fast‐moving picture speeds of 10 ppf or more compared with LCD TVs. Thus, this study confirms that OLED TVs, given their ultrafast response time characteristics, are superior in terms of moving picture images to LCD TVs. 相似文献
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Machine Intelligence Research - This paper proposes an image encryption algorithm LQBPNN (logistic quantum and back propagation neural network) based on chaotic sequences incorporating quantum... 相似文献
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A novel gel polymer electrolyte (GPE) which is based on new synthesized boron‐containing monomer, benzyl methacrylate, 1 m LiClO4/N,N‐dimethylformamidel liquid electrolyte solution is prepared through a one‐step synthesis method. The boron‐containing GPE (B‐GPE) not only displays excellent mechanical behavior, favorable thermal stability, but also exhibits an outstanding ionic conductivity of 2.33 mS cm?1 at room temperature owing to the presence of anion‐trapping boron sites. The lithium ion transference in this gel polymer film at ambient temperature is 0.60. Furthermore, the symmetrical supercapacitor which is fabricated with B‐GPE as electrolyte and reduced graphene oxide as electrode demonstrates a broad potential window of 2.3 V. The specific capacitance of symmetrical B‐GPE supercapacitors retains 90% after 3000 charge–discharge cycles at current density of 1 A g?1. 相似文献
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锂离子电池(LIB)是日常生活中最常见的便携式储能设备。然而,传统的锂离子电池多使用液态电解质(LE),存在易泄漏、易燃易爆且有毒等危险,其安全性日益受到关注。与LE相比,凝胶聚合物电解质(GPE)安全性更好且其电化学性能最接近LE,成为近年来电解质方面的研究重点。本文综述了近年来国内外GPE在LIB方面的研究进展,总结了传统聚合物基质采用交联、共聚或共混改性以提高电解质电化学性能及改善安全性方面的研究,并介绍了可再生、可降解的高分子材料在LIB方面的应用,旨在为研究功能性更强的GPE及高性能电极材料的研究提供参考。 相似文献