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The increased concentration of CO2 due to continuous breathing and no discharge of human beings in the manned closed space, like spacecraft and submarines, can be a threat to health and safety. Effective removal of low concentration CO2 from the manned closed space is essential to meet the requirements of long-term space or deep-sea exploration, which is an international frontier and trend. Ionic liquids (ILs), as a widespread and green solvent, already showed its excellent performance on CO2 capture and absorption, indicating its potential application in low concentration CO2 capture. In this review, we first summarized the current methods and strategies for direct capture from low concentration CO2 in both the atmosphere and manned closed spaces. Then, the multi-scale simulation methods of CO2 capture by ionic liquids are described in detail, including screening ionic liquids by COSMO-RS methods, capture mechanism by density functional theory and molecular dynamics simulation, and absorption process by computational fluid dynamics simulation. Lastly, some typical IL-based green technologies for low concentration CO2 capture, such as functionalized ILs, co-solvent systems with ILs, and supported materials based on ILs, are introduced, and analyzed the subtle possibility in manned closed spaces. Finally, we look forward to the technology and development of low concentration CO2 capture, which can meet the needs of human survival in closed space and proposed that supported materials with ionic liquids have great advantages and infinite possibilities in the vital area. 相似文献
3.
以1-甲基咪唑和氯代正丁烷为原料,合成1-丁基-3-甲基咪唑氯盐离子液体;以醋酸锌[Zn(Ac)2]、硫酸锌(ZnSO4)和氯化锌(ZnCl2)为锌源,在1-丁基-3-甲基咪唑氯盐离子液体和丙氨酸体系中与硝酸铈反应,经水热合成法制备得到Ce掺杂的纳米ZnO。采用扫描电子显微镜(SEM)、紫外-可见光吸收光谱(UV-Vis)、X射线衍射仪(XRD)、X射线光电子能谱分析(XPS)和红外光谱(FT-IR)对产品进行表征。以亚甲基蓝(MB)为目标降解物,采用UV-Vis检测,考察了Ce掺杂的纳米ZnO的光催化活性。研究表明,焙烧温度对光催化的晶体结构和光催化活性产生较大的影响;2%Ce/ZnO、焙烧温度为500℃、催化时间为30 min、亚甲基蓝用量0.05 g、pH值为10时降解率可达99.5%以上。 相似文献
4.
针对SIFT描述子实时性差和传统二进制描述子对尺度、旋转和视角变化鲁棒性差的问题,本文通过优化采样模式和添加灰度差分不变量比较测试进行改进,提出了一种鲁棒性更高的二进制描述子。首先,设计了一种尺度关联、编号标记的采样模式;然后,旋转采样模式中各采样点到特定位置,确保描述子尺度、旋转不变性;接着,分析了采样点点对模式对描述子的影响,选择使用机器学习训练后的128对采样点对;最后,选择灰度值比较测试及梯度绝对值和比较测试构建二进制描述子。实验中采用DoG检测图像关键点,结果表明:本文提出的描述子在描述子构建和描述子匹配上比SIFT描述子分别快84%和67%;在有视角变化的图像匹配上,准确率比传统的二进制描述子高3%~5%,召回率平均要高30%以上。本文提出的特征点描述方法适用于时间要求高的图像匹配领域。 相似文献
5.
Gas/liquid mass transfer has been investigated using a stirred vessel gas/liquid contactor using non‐Newtonian media and carbon dioxide as absorbent and gas phase, respectively. The volumetric mass transfer coefficients at different operational variables have been determined. Non‐Newtonian media (liquid phase) were prepared as aqueous solutions of sodium carboxymethyl cellulose salt. The influence of the rheological properties, polymer concentration, stirring rate, and gas flow rate on mass transfer was studied for these liquid phases. Kinematic viscosity and density experimental data were used to calculate the average molecular weight corresponding to the polymer employed. The Ostwald model has been used to fit the rheological behavior of aqueous solutions of the polymer employed as absorbent phase. Reasonably good agreement was found between the predictions of the proposed models and the experimental data of mass transfer coefficients. 相似文献
6.
论文从映射的角度,将哈希函数分为三类:严格哈希函数、计算哈希函数和实用哈希函数。在此基础上,根据二元域上二次方程x2 x c=0的部分不可解的性质,构造了一种计算哈希函数,它满足单向性和一一对应性,同时具有运算速度快的优点。 相似文献
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Results for various types of polar compounds in SRC-11 coal-derived liquids and other fuels were obtained by one or more of the three analytical methods: non-aqueous titration, i.r. spectroscopy and h.p.l.c. Practical aspects as well as precision, accuracy and assumptions necessary for effective application of each of the methods are discussed. H.p.l.c. is applicable to the widest variety of compound types, is the most rapid, most sensitive and shows the best promise for increased development and improvement. Application and development of these techniques is a logical step toward improving process monitoring, catalyst development, toxicological screening and general fuel analysis. 相似文献
9.
Modelling of Diffuse Interfaces with Temperature Gradients 总被引:1,自引:0,他引:1
The work is devoted to capillary phenomena in miscible liquids under the assumption that they have a constant and the same density. The model consists of the heat equation, diffusion equation, and the Navier-Stokes equations with the Korteweg stress. We study several configurations corresponding to the microgravity experiments planned for the International Space Station. The basic conclusion of the numerical simulations is that transient capillary phenomena in miscible liquids exist and can produce convective flows sufficiently strong to be observed experimentally. In particular, there exists a miscible analogue to the Marangoni convection where the temperature gradient is applied along the transition zone between two fluids. Convection also appears if, instead of the temperature gradient, the case where the width of the transition zone varies in space is considered. Finally, similar to the immiscible case, miscible drops move in a temperature gradient. 相似文献
10.
Cathy Lawson Douglas C. Montgomery 《Quality and Reliability Engineering International》2006,22(8):971-984
Variation exists in all processes. Significant work has been done to identify and remove sources of variation in manufacturing processes resulting in large returns for companies. However, business process optimization is an area that has a large potential return for a company. Business processes can be difficult to optimize due to the nature of the output variables associated with them. Business processes tend to have output variables that are binary, nominal or ordinal. Examples of these types of output include whether a particular event occurred, a customer's color preference for a new product and survey questions that assess the extent of the survey respondent's agreement with a particular statement. Output variables that are binary, nominal or ordinal cannot be modeled using ordinary least‐squares regression. Logistic regression is a method used to model data where the output is binary, nominal or ordinal. This article provides a review of logistic regression and demonstrates its use in modeling data from a business process involving customer feedback. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献