大气压针板介质阻挡放电中微流注、电晕和辉光放电相互转换研究（英文）

To discuss the modes of dielectric barrier discharge(DBD) between needle-to-plane electrodes in air,DBD is generated and observed on a needle-to-plane device at atmospheric pressure air.Fast images of the DBD are taken by using a charge couple device(CCD) cinema with a macro lens,while the electrical and photo-electricity waveforms of the DBD are recorded.The current waveforms show that under an applied voltage of 3 kV,there are numerous short current pulses in both positive and negative half-periods of discharges.However,under 6 kV,there are still the numerous short current pulses in the positive half-periods,but only one wide current pulse in each negative half-period.This difference is also found in the photoelectric signals.The streamer,corona and glow discharges are observed from the images of the discharges at different applied voltages.The structure of glow discharge in the negative period is exactly the same as that of the low pressure glow discharge.However,in the positive period of discharge there is always a streamer.In the negative period of discharge,while the applied voltage increases,the transition from corona to glow discharge is observed.The progress of a transition between streamer and glow discharge at 6 kV during one period is analyzed.The glow discharge appearance is determined by two factors: the discharge current is limited to a certain extent by the dielectric layer; the charges deposited on the dielectric layer during the last half period enhance the intensity of the electric field.At an insufficient applied voltage,the cathode drop leads to no glow discharge,but Trichel pulses.     

在共面介质阻挡放电中大气压等离子体射流的特性(英文)

Non-thermal plasma jet at atmospheric pressure has recently attracted lots of attention because of its applications in plasma bullet or plasma plume.Thus,we studied on generating plasma jet by coplanar dielectric barrier discharge in a device driven by sinusoidal voltage.The processes of plasma discharges in both positive and negative half cycles were recorded using a high-speed ICCD(intensified charge-coupled device)camera;based on the results we estimated the velocity of plasma propagation,and investigated the influence of gas flow on the plasma development.It is shown that the plasma bullets,which have velocity in the order of 103～104m/s,exist only outside the cathode.APPJ(atmospheric pressure plasma jet)is created by the electron beam from the cathode,and then sustained by a strong radial electric field near and outside the cathode.The gas flow influences the APPJ length in air but not the APPJ discharge,while the discharge is affected significantly by the applied voltage.     

SF6对介质阻挡放电臭氧生成的影响（英文）

The influence mechanism of a small amount of SF6 on ozone generation in oxygen or air discharge is investigated.Some results are obtained by probing into the number of the high-energy electrons,which have the sufficiency energy for generating ozone.Introducing a small amount of SF6 into oxygen sharply decreases the number of high-energy electrons,because the electron density decreases sharply while the mean electron energy remains constant due to higher breakdown voltage and lower discharge power,and some high-energy electrons are consumed by the excitation and attachment of SF6.In contrast,when a small amount of SF6 is added into dry air discharge,despite the consumption of the excitation and attachment of SF6,the number of high energy electrons increases sharply,which is attributed to the higher mean electron energy and electron density resulted from higher breakdown voltage and discharge power.When the volume fraction of SF6 increases from 0 to 2.22%,the ozone mass concentration and the ozone yield increase by 45.7% and 29.7%,respectively.Therefore,though the oxygen source should avoid the presence of SF6,adding a small amount of SF6 can improve the ozone mass concentration and the efficiency of ozone generation.     

中频脉冲直流磁控放电等离子体仿真（英文）

Pulsed magnetron sputtering in the mid-frequency range(5~350 kHz) has recently become a promising industrial technique for the deposition of high-quality films.In order to study the plasma properties in a pulsed DC magnetron,a two-dimensional self-consistent particle model is developed,and the temporal and spacial evolution of electrons and ions in discharge space are simulated.In these simulations,the magnetic field is calculated by finite element method,and the plasma is modeled by PIC/MCC(Particle-In-Cell,Monte Carlo Collision) method.The plasma density and the electric potential in the pulse-on and the pulse-off phases are preassigned,and then the temporal evolution of plasma close to the cathode and the substrate is analyzed.It is found that electrons accumulate close to the cathode in the pulse-off phase more than in the pulse-on phase,and hence the positive particles at the target are neutralized and the electric arc is suppressed.Moreover,more energetic ions accumulate close to the substrate.They bombard the film,and this enhances the film’s quality.     

大气压下重复频率纳秒脉冲气体放电中X射线的辐射特性(英文)

Pulsed discharges can generate high power densities and high equivalent electric fields in plasma to emit X-rays,which is closely related to discharge mechanism.In this paper,discharge characteristics and X-ray emission of typical nanosecond-pulse discharges(corona,diffuse,spark or arc)are reviewed.Especially,the diffuse discharges are observed at pulse repetition frequencies up to 1 kHz.Factors influencing the discharge characteristics and X-ray emission are analyzed,such as the gap spacing,parameters of the applied pulse(amplitude,pulse repetition frequency),anode and cathode materials,and curvature radius of cathode.It is concluded that the maximum X-ray intensity is obtained in a diffuse discharge,and the X-ray intensity is affected by the pulse repetition frequency,applied voltage,anode material,and curvature radius of cathode.For example,X-ray intensity increases with the pulse repetition frequency and the atomic numbers of the anode material,but it decrease with the increase of curvature radius.It is also shown that the cathode material has no obvious influence on the X-ray intensity.     

大气压下高压亚微秒脉冲激励产生的介质阻挡放电的实验分析(英文)

An experimental device is used to study the characteristics of dielectric barrier discharge(DBD)plasma excited by high voltage sub-microsecond pulse power in atmospheric air.Glass,polytetrafluoroethene(PTFE)and plexiglass are used as dielectric barrier materials.Comparatively homogeneous discharge is obtained within 130 mm diameter area in atmospheric air using the three dielectric materials with gap distances of 4.5 mm,6.5 mm and 6.5 mm,respectively.There is no filamentary discharge observed by naked eyes or by camera with the exposure time of 0.25 s.Gas gap voltage,discharge current,discharge power density,etc.are calculated by using Liu’s equivalent circuit model for pulsed DBD.These parameters are used to study the DBD characteristics.Typically,current varies from tens of amperes to hundreds of amperes in atmospheric air DBD excited by sub-microsecond pulses.The peak power can reach to MW order of magnitude.The average power surface density of 1.0 W/cm2and the average electron density of 1011cm 3can also be obtained in the discharge.Rotational and vibrational temperatures,approximately 400 K and 2 650 K,respectively,are obtained by using the emission spectrum of the discharge.This is the basic work performed for a better understanding of the characteristics of atmospheric air DBD plasma excited by high voltage sub-microsecond pulsed power source.     

直流电场下低密度聚乙烯纳米介质空间电荷特性的数值分析(英文)

The dynamic characteristics of space charge in nanocomposite of low-density polyethylene (LDPE) mixed with inorganic nano- fillers. Different from previous qualitatively theoretical works, we investigated the influence of trap depth, trap volume charge density and injection barrier height on the space charge and the electric field distribution in the nanocomposite under a DC external electric field (100 MV/m) systematically and quantificationally, through numerical simulations based on a bipolar charge transport model. The simulation re- sults showed that, the increase of trap depth would severely distort the balanced electric field distribution with the highest and the lowest electric field of 119 MV/m and 47 MV/m, respectively. It is concluded that the introduction of nanofillers creates more deep traps, which would block space charges by capturing most of them in the vicinity of electrode and hence reduce the local electric field largely. Further theoretical analysis of the simulation indicates that both the high permittivity and the low local electric field of the nanocomposite contri- buted to the increase of injection barrier height, and almost no charge could overcome an injection barrier higher than 1.25 eV. At last, a mechanism of space charge suppression in the LDPE nanocomposite was presented.     

局部放电射频信号与其视在放电量的关联分析(英文)

Radio frequency(RF) measurement has become a hot issue for partial discharge detection.However,its application is hampered by the difficulty to establish a relationship between the RF measurements data and apparent discharge quantity.In this paper,on the basis of an experimental model of metal protrusion,the relationship between the results of RF measurement and pulse current method(IEC 60270) was investigated.The energy,double integration,peak voltage,peak-peak voltage and the area of RF signals were plotted versus either the apparent discharge quantity or the square of the apparent discharge quantity in order to evaluate the optimal regression curve.At the same time,the impact of voltage and the distance between protrusion and plate were also investigated.The results indicate that the optimal match to a linear regression curve can be gained by plotting the RF signal energy versus the square of the apparent discharge quantity.The variation of voltage has no significant impact on the regression curve;that is,data from different voltages match one line.However,when the distance between protrusion and plate is changed,the slope of the regression curve changes accordingly;the same energy corresponds to a bigger discharge quantity.The results are significant enough to be applied in the estimation of the discharge quantity by measuring RF partial discharge signals.     

惰性气体对氧气介质阻挡放电臭氧生成的影响(英文)

This paper reports the results of an experimental study of the effect of inert gases He,Ar and Kr on ozone generation in a Dielectric Barrier Discharge(DBD) fed by pure oxygen.The chemical reaction mechanisms related to the process of ozone generation are discussed.The experimental results show that ozone concentration decrease with decreasing oxygen content in all He+O2,Ar+O 2 and Kr+O 2 mixtures mainly owing to the decrease of oxygen content.The conversion ratio of oxygen into ozone increases with increasing oxygen content in He+O2 mixtures,but the addition of Ar and Kr can improve the conversion ratio due to the increase of free electrons density and excited oxygen molecules required for ozone formation through ionization and Penning effect.The effect of Kr is more significant for the lower first ionization energy of metastable state compared with other gases.It is probable that the ozone concentration,and ozone production efficiency increase with Kr addition when the reduced electric field and mean electron energy are high enough.     

甚高频对大气压Ar/SiH4/H2混合等离子体粒子密度分布影响的数值模拟（英文）

To improve the microcrystalline silicon thin film deposition in quality and to increase its microcrystalline silicon content,we numerically investigated the characteristics of homogeneous discharges in hydrogen diluted silane and argon mixed gases at atmospheric pressure using a two-dimensional fluid model.The model takes into account the primary processes of excitation and ionization,sixteen reactions of radicals with radicals in silane/hydrogen/argon discharges,so this model can adequately describe the discharge plasma.The effects of very high frequency(VHF)excitation on the electron density in such discharges are analyzed.The simulation results show that the electron density does not linearly vary with the excitation frequency within from 90150 MHz.he maximum value occurs at an appropriate excitation frequency i.e.the transition frequency.Increasof the excitation frequency would effectively increase the electron density before the transition frequency,but decreases the density afterwards.is.Moreover,the densities of involved particle species,including H2+,H,Ar*,Ar+,SiH3+,SiH3,SiH3,SiH2are closely interrelated.     

不均匀电场下加压气体中弥散放电和火花放电的形成(英文)

Diffuse and spark discharges are formed and studied during breakdowns with nonuniform electric field in nitrogen,air,and argon at elevated pressures and pulse repetition frequency of 400 Hz.Negative-polarity voltage pulses of the amplitude 20 kV,width at the base of 15 ns and rise time of 2 ns are applied to the electrode with a small radius of curvature.In the conditions of generation of runaway electron beams and X-rays,a CCD camera records the time of the diffuse discharge formation and its duration prior to its transition to a spark one.In all three gases,the diffuse discharge is formed during the time not exceeding 1 ns,when the bright spots appear on cathode in argon and air resulting in the beginning of the spark channel propagation.     

闪电放电通道的等离子体特性（英文）

The plasma characteristics of a lightning discharge channel are reviewed.The spectrum of the natural lightning is investigated by employing the slit-less spectrograph.It is found that the spectrum characteristics are closely related to the intensity of the lightning discharge.The lines in the lightning spectrum are classified into essential lines and characteristic lines,according to the characteristics of lightning spectra with different intensities.The characteristics of the lightning channel and the radiation of the lighting plasma are analyzed in the visible and infrared regions.It is shown that,the visible spectrum of lightning is determined by the radiation generated from the early stage to the development of lightning,while the near-infrared spectrum is determined by the radiation generated after current of lightning reaches the peak.The channel temperature and the electron density are calculated using the information obtained from the lightning spectrum.Both the temperature and the density decrease with the increasing length of lightning channel.Moreover,X-rays and neutrons are produced in the process of lighting mainly due to the pinch effects.     

高压下非均匀电场中局放机理的建模(英文)

Partial discharges in air in non-uniform electric field occur in surroundings made of high curvature elements.The equivalent electrode system,needle-plane refers both to external components of high voltage insulating systems and to micro sharpness in the internal structure of those systems.The ionization zone,accumulation of space charge and formation of corresponding current pulses depend on electrode configuration,voltage level,pressure,temperature and humidity of air.The assessment of pressure influence on discharge mechanism in non-homogenous electric field has been performed on the basis of empirical density distributions of discharge charges at different voltage levels,electrode distance,curvature of high voltage electrode and taking into account solid dielectric barrier in serial configuration.The measurement results obtained at variable voltage level yield the influence of electric field strength in the needle electrode zone.While increasing voltage,a deviation from normal distribution may be observed that reveals other forms of discharge.     

大气压氦气与氩气等离子体射流形成机理的对比研究(英文)

To compare the formation mechanisms of He and Ar atmospheric pressure plasma jets(APPJs),an intensified charge-coupled device(ICCD)are utilized to observe the dynamic process of APPJ.The experimental results show that,He APPJ is first ignited,which is independent of the dielectric barrier discharge(DBD)between the two wrapped electrodes when the high voltage placed at the downstream.The intensity and APPJ length under positive discharge pulses are bigger than that under negative discharge pulses due to the space charge effect.The He APPJ is formed by the DBD development when the high-voltage electrode placed at the upstream side of tube.However,the plasma plume in Ar APPJ is formed by the propagation of DBD whatever the high-voltage electrode is arranged on upstream or downstream side of ground electrode.The difference in formation mechanism between He and Ar APPJs is mainly caused by the gas properties.Moreover,during the discharges,Ar tends to lead to thermal instability and electron Maxwellian instability.     

Effect of Barrier Materials on Discharge Properties in Air at Low Pressure

Dielectric barrier discharge(DBD) is widely investigated in order to obtain uniform low-temperature plasma.Many studies have proved that some barrier materials,especially electrets,can improve the uniformity of discharge.It is regarded as an available way to get atmospheric pressure glow discharge(APGD).In this paper,discharge forms with 4 different barrier materials(alumina,quartz,PTFE and PET) are investigated,and the transition of discharge form depending on the air pressure are recorded to estimate the influence of barrier materials on discharge.By using electrets as barrier materials,homogeneous discharges can be obtained in a more wide pressure range.Under the same experimental conditions,discharges with electrets are more uniform or have larger uniform areas due to the storage and desorption of charges on the surface of electrets.The electrons deposited in the surface layer can be released on next half cycle when the polarity of the applied voltage changes,and provide a number of seed electrons,which makes the discharge more homogeneous.The capacitance and the permittivity of barrier materials have no effect on the discharge form directly.     

外电场及预电离对大功率脉冲氙灯放电等离子体特性的影响(英文)

This work is devoted to experimentally study the characteristics of discharge plasma in high power xenon flashlamps.In the experiments,plasma channel profiles are captured by using a high speed CCD camera,and the radiation energy of the flashlamp is obtained by a pyroelectric energy meter.Voltage and current curves are recorded to shed light on the plasma characteristics.With these diagnostic methods,typical factors influencing the evolution process of plasma channel are studied,including the external electric field and the pre-ionization.The electric potential distribution in the flashlamp influence the plasma channel characteristics the most significantly.The plasma channel pattern for the cases with grounded wires is different from that with ungrounded metal wires.When the wire is ungrounded,it is the coupling voltage between the metal wire and the flashlamp that influences the development of plasma channel.In terms of radiation efficiency,it is proven that there is an optimal interval within 200～300μs between the pre-ionization pulse and the main pulse.     

氩气与氨气混合下的大气压介质阻挡放电(英文)

In this paper,the influence of ammonia admixture on argon discharge properties is investigated.Electrical measurements,as well as ten-nanoseconds-exposure photographs taken by an intensified charge-coupled device(ICCD)camera,are employed to confirm the existence of atmospheric pressure glow discharge(APGD)in Ar/NH3mixture.The breakdown voltage and transition voltage between APGD and filamentary discharge are studied at various ammonia concentrations.The results show that a small amount of NH3can lead to APGD due to the Penning ionization of NH3molecules by metastable argon,and the breakdown voltage increases with the growth in NH3concentrations owing to the electronegative feature of NH3.The optical emission spectrum of Ar/NH3APGD is analyzed.Besides,gas temperature is estimated at 327 K by the diagnoses of the OH(A-X)(0,0)band of the spectrum.     

裸露金属电极中的亚微秒脉冲常压辉光放电（英文）

In order to better understand the physical mechanism of sub-microsecond pulsed glow discharge with bare metal electrodes,using a one-dimensional self-consistent fluid model,the properties of the discharge at atmospheric pressure are numerically studied.The results show that,a discharge without dielectric layers,i.e.a barrier free discharge,is extinguished only with the decrease of the applied voltage.Only one positive discharge event occurs at the slope of the pulsed voltage.A stable glow of barrier free discharge can be achieved only in short durations of the pulsed voltage.The barrier free discharge always starts with a subnormal glow discharge and then evolves into a normal glow discharge.Moreover,to control the discharge stabilization better,the effects of pulse repetition frequency,pulse duration,rising(front) and falling(slope) times on the discharge characteristics are investigated systematically.It is found that the discharge is comparatively more sensitive to the repetition frequency and the pulse duration,while little affected by the rising and falling times.     

电晕放电脉冲电流波形和相位分布的测量、分析与仿真(英文)

Partial discharge(PD) is one of the most important phenomenon in high voltage insulations.In most cases, the appearance of partial discharges is related to insulation defects.Understanding partial discharges is important for diagnosis on insulation condition.Corona discharges appear when extremely high electric field appears on the conductor surface exceeding the electric field strength of the gas.The high electric field may occur at around protrusion with very sharp tip.This paper reported a holistic approach of corona discharge investigation.The needle-plane electrode system was used.The medium between the electrodes was air.The needle was made from steel with radius of curvature of 3μm(Ogura needle).Sinusoidal as well as triangular applied voltages were used.The waveform of the corona discharges was measured using a digital oscilloscope.The corona discharge pulses were measured using a phase-resolved PD measurement system.The system was able to measure the magnitude(q) and phase angle position(φ) of each PD pulses,as well as the number of discharge pulses(n).The role of applied voltage was investigated using phase-resolved analysis of corona discharge pulses through pulse sequence,pulse magnitude and pulse number analysis. Experimental results indicated that corona discharge current waveform was an impulse with rise time of about several ns and the impulse width of about 100 ns.The Fast Fourier Transform analysis indicated that the corona discharge current waveform had several spectrum peaks at frequency of 7.8 MHz,85.9 MHz,109.4 MHz and 195.3 MHz.The experimental results also showed that discharge pulses were concentrated around the peak of applied voltage for both sinusoidal and triangular voltages.The discharge magnitude,as well as its probability of occurrence,was strongly dependent on the instantaneous applied voltage.The shape ofφ-n,as well asφ-q-n PD patterns,were strongly reflected by the shape of applied voltage.In order to get deep understanding of the corona discharge,by utilizing results of the phase-resolved analysis,electrical equivalent circuits of corona discharges were proposed.The electrical equivalent circuit contained capacitances and a spark gap.For deeply understanding of PD phenomenon,computer simulation was done by using the proposed electrical equivalent circuits.The similarity of the measured and simulated PD patterns was assessed by comparing measured and simulated theφ-q-n andφ-n PD patterns.The results indicated that simulated PD patterns similar to those obtained from experiment.