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《International Journal of Hydrogen Energy》2022,47(5):2926-2935
Development of highly efficient and cheap electrocatalysts towards the hydrogen evolution reaction (HER) is of great importance for electrochemical water splitting. Herein, hybrid Cu/NiMo-P nanowires on the copper foam were successfully fabricated via a simple two-step method. The hierarchically structured Cu/NiMo-P exhibits large surface areas and rapid electron transfer ability, leading to enhanced catalytic activity. The as-prepared Cu/NiMo-P electrodes need overpotentials of 34 mV and 130 mV to obtain 10 mA cm?2 for HER in acidic and alkaline solutions, respectively. Density functional theory (DFT) calculations reveal that the Cu/NiMo-P hybrid has a more thermo-neutral hydrogen adsorption free energy and enhanced charge transfer ability as well. 相似文献
3.
Jean-Claude Malela-Majika Sandile Charles Shongwe Olatunde Adebayo Adeoti 《Quality and Reliability Engineering International》2021,37(8):3314-3322
The sensitivity of a monitoring scheme depends on many factors including the variance of the charting statistic which is very important in the computation of the control limits. This paper discusses the computation of the variance of the recently proposed hybrid homogeneously weighted moving average (HHWMA) scheme which was based on an incorrect assumption. The correct variance is used to evaluate the run-length characteristics of the HHWMA scheme. It is observed that the incorrect variance has a significant impact on the sensitivity (or performance) of the HHWMA scheme. 相似文献
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Iqbal Ahmad Syed Mujtaba Shah Muhammad Nadeem Zafar Muhammad Naeem Ashiq Wei Tang Uzma Jabeen 《Ceramics International》2021,47(3):3760-3771
Ferrites are materials of interest due to their broad applications in high technological devices and a lot of research has been focused to synthesize new ferrites. In this regard, an effort has been devoted to synthesize spinel Pr–Ni co-substituted strontium ferrites with a nominal formula of Sr1-xPrxFe2-yNiyO4 (0.0 ≤ x ≤ 0.1, 0.0 ≤ y ≤ 1.0). The cubic structure of pure and Pr–Ni co-substituted strontium ferrite samples calcinated at 1073 K for 3 h has been confirmed through X-ray diffraction (XRD). Average sizes of crystallites (18–25 nm) have been estimated from XRD analysis and nanometer particle sizes of synthesized ferrites have been further verified by scanning electron microscopy (SEM). SEM results have also shown that particles are mostly agglomerated and all the samples possess porosity. It has been observed that at 298 K, the values of resistivity (ρ) increase, while that of AC conductivity, dielectric loss, and dielectric constants decrease with increasing amounts of Pr3+ and Ni2+ ions. The values of dielectric parameters initially decrease with frequency and later become constant and can be explained on the basis of dielectric polarization. Electrochemical impedance spectroscopy (EIS) studies show that the charge transport phenomenon in ferrite materials is mainly controlled via grain boundaries. Overall, synthesized ferrite materials own enhanced resistivity values in the range of 1.38 × 109–1.94 × 109 Ω cm and minimum dielectric losses, which makes them suitable candidates for high frequency devices applications. 相似文献
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基于传统易碎薄板机械手位置伺服控制系统稳定性低、自动化分拣效率低等不足,设计了一种基于笛卡尔坐标式的气动码垛机器手和位置伺服稳定性控制系统。首先,设计并介绍笛卡尔坐标式码垛机械手的基本组成结构,对机械手末端吸盘气动回路控制系统进行设计和分析;然后分别对机械手X、Y、Z三个方向的伺服电机控制原理进行分析并设计了一种位置伺服系统的前馈自适应控制算法;最后,将传统位置闭环PID算法和前馈自适应控制算法进行位置跟踪稳定性对比试验。实验结果表明该笛卡尔坐标式的气动码垛机器手和位置伺服稳定性控制系统设计合理,满足实际生产要求。 相似文献
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CO2捕集作为温室气体排放控制的有效手段已成为重要研究课题。作为新兴捕集技术之一,低温CO2捕集因产品纯度高、无附加污染等优势受到关注。然而,该技术能耗和捕集率对于气体中CO2浓度十分敏感,对于高CO2浓度气体可获得较高的CO2捕集率和较低能耗水平。基于此,本文提出了耦合膜分离的新型CO2低温捕集系统,通过膜材料选择渗透性实现待捕集气体CO2浓度主动调控,并在最优浓度下进行CO2低温捕集。首先基于不同传统低温捕集系统特点,对比分析了不同耦合系统模式,从而确定了最优耦合系统结构。针对最优耦合系统进行了运行参数优化,并分别基于实现系统捕集能耗最低与捕集率最高的目标,获得了膜渗透侧CO2浓度与进气CO2浓度间的关系式,为该耦合系统中膜组件选型提供指导。研究表明,本文提出的耦合系统捕集能耗为1.92MJ/kgCO2,相比于传统单一低温系统捕集能耗可降低16.5%。 相似文献
9.
Chuntao Lan Haiyang Zou Longfei Wang Meng Zhang Shuang Pan Ying Ma Yiping Qiu Zhong Lin Wang Zhiqun Lin 《Advanced materials (Deerfield Beach, Fla.)》2020,32(47):2005481
Despite recent rapid advances in metal halide perovskites for use in optoelectronics, the fundamental understanding of the electrical-poling-induced ion migration, accounting for many unusual attributes and thus performance in perovskite-based devices, remain comparatively elusive. Herein, the electrical-poling-promoted polarization potential is reported for rendering hybrid organic–inorganic perovskite photodetectors with high photocurrent and fast response time, displaying a tenfold enhancement in the photocurrent and a twofold decrease in the response time after an external electric field poling. First, a robust meniscus-assisted solution-printing strategy is employed to facilitate the oriented perovskite crystals over a large area. Subsequently, the electrical poling invokes the ion migration within perovskite crystals, thus inducing a polarization potential, as substantiated by the surface potential change assessed by Kelvin probe force microscopy. Such electrical-poling-induced polarization potential is responsible for the markedly enhanced photocurrent and largely shortened response time. This work presents new insights into the electrical-poling-triggered ion migration and, in turn, polarization potential as well as into the implication of the latter for optoelectronic devices with greater performance. As such, the utilization of ion-migration-produced polarization potential may represent an important endeavor toward a wide range of high-performance perovskite-based photodetectors, solar cells, transistors, scintillators, etc. 相似文献
10.
Olatunde Adebayo Adeoti Sunday Olawale Koleoso 《Quality and Reliability Engineering International》2020,36(6):2170-2186
Several modifications and enhancements to control charts in increasing the performance of small and moderate process shifts have been introduced in the quality control charting techniques. In this paper, a new hybrid control chart for monitoring process location is proposed by combining two homogeneously weighted moving average (HWMA) control charts. The hybrid homogeneously weighted moving average (HHWMA) statistic is derived using two smoothing constants λ1 and λ2 . The average run length (ARL) and the standard deviation of the run length (SDRL) values of the HHWMA control chart are obtained and compared with some existing control charts for monitoring small and moderate shifts in the process location. The results of study show that the HHWMA control chart outperforms the existing control charts in many situations. The application of the HHWMA chart is demonstrated using a simulated data. 相似文献