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1.
《International Journal of Hydrogen Energy》2022,47(12):7836-7845
Catalyst samples for CH4 decomposition were prepared from red mud (RM) by an acid-leaching neutralization precipitation approach. Water-washing the resultant precipitates multiple times, followed by drying at 105 °C and calcination at 500 °C, resulted in a threshold of residual Na2O, equivalent to 96% Na2O removal. Drying the precipitate at a higher temperature of 200 °C, followed by repeated water washing, provided a deeper Na2O removal of 99% and made the resultant samples more active for the targeted reaction. Subsequently, four catalyst samples with a simulated red mud composition and NaOH contents from 0 to 0.3 wt% were prepared and the catalytic test results revealed that the Na2O remaining in the RM-derived catalysts did not only inhibit their activation in CH4 but also lower their maximal activities for CH4 decomposition. Finally, two catalysts with the same simulated red mud composition and their Na impregnated respectively on Fe2O3 and a mixture support of Al2O3-SiO2-TiO2 were prepared and tested to explore the effect of Na distribution on the activation behavior of RM-derived catalysts for CH4 decomposition. The activity testing results showed that it was the Na residual dispersed on iron oxides in the RM-derived samples to significantly inhibit the activation of CH4 decomposition. 相似文献
2.
Qian Wu Xiangmei Liu Bo Li Lei Tan Yong Han Zhaoyang Li Yanqin Liang Zhenduo Cui Shengli Zhu Shuilin Wu Yufeng Zheng 《材料科学技术学报》2021,67(8):70-79
Pathogens pose a serious challenge to environmental sanitation and a threat to public health.The frequent use of chemicals for sterilization in recent years has not only caused secondary damage to the environment but also increased pathogen resistance to drugs,which further threatens public health.To address this issue,the use of non-chemical antibacterial means has become a new trend for environmental disinfection.In this study,we developed red phosphorus nanoparticles(RPNPs),a safe and degradable photosensitive material with good photocatalytic and photothermal properties.The red phosphorus nanoparticles were prepared using a template method and ultrasonication.Under the irradiation of simulated sunlight for 20 min,the RPNPs exhibited an efficiency of 99.98%in killing Staphylococcus aureus due to their excellent photocatalytic and photothermal abilities.Transmission electron microscopy and ultraviolet–visible spectroscopy revealed that the RPNPs exhibited degradability within eight weeks.Both the RPNPs and their degradation products were nontoxic to fibroblast cells.Therefore,such RPNPs are expected to be used as a new type of low-cost,efficient,degradable,biocompatible,and eco-friendly photosensitive material for environmental disinfection. 相似文献
3.
《Ceramics International》2022,48(13):18793-18802
The luminescence center energy transfer, crystal field strength, and covalency are limited by the crystal structure of the host and subsequently affect the luminescence efficiency, color, and intensity. Here, we report an excellent red phosphor BaLaLiWO6:0.40Eu3+ and the dependence between symmetry and luminous performance. A model for changing symmetry is drawn by analyzing the Coulomb potential and structure for the application of a double-perovskite phosphor BLLWO: Dy3+, Eu3+ in white light LEDs. The addition of Dy3+/Eu3+ makes the W-O bond formed by the B-site and oxygen ion longer and the Li-O bond shorter, and the difference between the eight octahedral around the A-site is reduced, increasing the symmetry of the A-site. Local symmetry was successfully modulated by changing the Eu3+ concentration to control the Y/B ratio of Dy3+ and the R/O ratio of Eu3+ and smoothly achieved (0.382, 0.373) warm white light color coordinate. The phosphor has excellent thermal stability and still has 92.3% intensity at 475 K. The above results show that the wavelength composition of the luminescence is tunable by changing the symmetry of the environment in which the doped ions are located. It applies to single hosts for the regulation of white light emission. 相似文献
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High dimensionality in real-world multi-reservoir systems greatly hinders the application and popularity of evolutionary algorithms, especially for systems with heterogeneous units. An efficient hierarchical optimization framework is presented for search space reduction, determining the best water distributions, not only between cascade reservoirs, but also among different types of hydropower units. The framework is applied to the Three Gorges Project (TGP) system and the results demonstrate that the difficulties of multi-reservoir optimization caused by high dimensionality can be effectively solved by the proposed hierarchical method. For the day studied, power output could be increased by 6.79 GWh using an optimal decision with the same amount of water actually used; while the same amount of power could be generated with 2.59 × 107 m3 less water compared to the historical policy. The methodology proposed is general in that it can be used for other reservoir systems and other types of heterogeneous unit generators. 相似文献
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三峡三期工程主坝大体积混凝土内部温度控制 总被引:2,自引:2,他引:0
三峡右岸三期工程施工中,为了有效控制坝体大体积混凝土内部温升,采取了高温季节使用预冷混凝土浇筑、控制混凝土出机口温度及浇筑温度、对混凝土内部人工通水进行初冷、中冷和后冷等措施。三峡三期工程大坝混凝土内部温度没有出现超标现象,混凝土温控工作取得了良好的效果。 相似文献
7.
本文介绍了三峡工程进入2002年后工程建设的新特点,并对工程下一步两个重点项目三期截流和碾压混凝土围堰的技术难点和工期安排做了深入分析。另外,作者根据国家电力体制改革的重要内容,以及中国三峡总公司自身情况,对公司未来的可持续发展之路亦做了深入探讨。借助中国三峡总公司的品牌优势和资本实力,吸收其它形式的能源,优化能源结构;进一步降低工程造价,提高三峡电价在电力市场的竞争力;依靠科学管理,实现电力生产利润最大化,深化内部改革等措施,促进中国三峡总公司可持续发展。 相似文献
8.
三峡水库减淤增容调度方式研究——多汛限水位调度方案 总被引:8,自引:0,他引:8
本文建议在汛期中小流量时(Q<35000m3/s),将坝前水位维持在148~151m;出现汛情且流量更较大后,将坝前水位降低到143m;入库流量大于35000m3/s且短期预报将出现大于十年一遇洪水时,预泄洪水到135m.按这一调度,汛期约80%时间可以维持在较高水位,一般洪水期。汛限水位143m不影响坝区通航,135m水位迎洪可大量增加防洪库客。到100年后可减淤30亿m3,增加防洪库容约40亿m3.变动回水区减淤40%,优化了坝区水沙搭配,可改善通航条件。降低库区洪水位,缓解防洪与移民的矛盾。可对发电带来较大好处:提高发电效益,减少粗沙过机。初期水库排沙比大于原方案,可减轻下游冲刷。同时,可减小三峡汛初泄水与鄱阳湖防洪的矛盾。 相似文献
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