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《International Journal of Hydrogen Energy》2022,47(49):21231-21240
To explore the feasibility and related mechanism of MFC biosensor for wastewater detection under the action of combined heavy metals. Cyclic voltammetry (CV) and scanning electrochemical impedance spectroscopy (EIS) were used to explore the related bioelectrochemical process. The response of the reactor to single/combined heavy metals, low/high heavy metal concentrations, and the differences in ohmic resistance (Rs) and charge transfer resistance (Rct) were investigated using Ni as the core heavy metal and the combined action of Cd, Cu and Zn. The results indicated that there was a linear relationship between the concentration and output voltage of the MFC biosensor under the action of combined heavy metals (R2 = 0.8803–0.973). However, the internal resistance (Rint) of the MFC biosensor under the action of single heavy metal was far less than that of the combined heavy metal group, and the power density (19.849 W m?3) was 4 times that of the combined heavy metal group (3.109–4.589 W m?3). The Rs of the biosensors in the combined heavy metal group were 0.868Ω and 0.860, which were higher than 0.768Ω of the single heavy metal sensor. With the increase of the concentration of heavy metals in the influent, the increase of Rct was more obvious in the combined group, while the Rs in the single group significantly increased (P < 0.05). The results imply that it is possible for MFC biosensors to be used in the detection of actual water polluted by various heavy metals, but the biosensor performance is mainly limited by Rct, which needs to be further improved. 相似文献
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甫沙4井位于塔里木盆地塔西南坳陷昆仑山前冲断带的柯东构造带上,北部和东部分别发育有柯克亚和柯东1井油气田。为研究甫沙4井原油来源与充注过程,对原油样品和连续抽提后的含油砂样各组分(游离态、束缚态、包裹体)进行GC、GC?MS和 GC?IRMS分析,与柯克亚凝析油气田油样进行油—油对比。结果表明:甫沙4井晚期充注原油组分具有C29?32重排藿烷、重排甾烷和Ts相对含量高,C27?29甾烷ααα 20R分布呈反“L”型,以及正构烷烃单体碳同位素值较低等特征,与柯克亚凝析油气田来源于二叠系普司格组(P2?3p)烃源岩的主体原油(I类)地球化学特征一致。而早期充注的原油组分具有重排藿烷、重排甾烷和Ts相对含量较低,C27?29甾烷ααα 20R分布呈“V”型,以及正构烷烃单体碳同位素值较高等特征,与柯克亚凝析油气田来源于中—下侏罗统湖相泥岩的II类原油地球化学特征一致。甫沙4井经历3个阶段成藏过程:①在上新世,二叠系烃源岩于生油晚期阶段生成的I类原油运移至柯克亚构造带或柯东构造带深部形成油藏;②在更新世早期,侏罗系烃源岩于生油早—中期生成的II类原油运移至甫沙4井白垩系储层;③在第四纪,强烈的构造作用使深部I类原油沿断裂调整进入甫沙4井白垩系储层。最终造成甫沙4井白垩系储层II类原油先充注,I类原油后充注的特殊现象。 相似文献
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《Journal of the European Ceramic Society》2022,42(3):1014-1022
In this work we have investigated the effect of the solvent during the processing of SrFe12O19 platelet-based permanent magnets by cold sintering process (CSP) plus a post-thermal treatment. Several organic solvents: glacial acetic acid, oleic acid and oleylamine have been analyzed, optimizing the CSP temperatures at 190?270 °C, under pressures of 375?670 MPa and 6?50 wt% of solvent. Modifications in the morphological and structural properties are identified depending on the solvent, which impacts on the magnetic response. Independently of the solvent, the mechanical integrity of ferrite magnets obtained by CSP is improved by a post-annealing at 1100 °C for 2 h, resulting in relative densities around 92 % with an average grain size of 1 μm and a fraction of SrFe12O19 phase >91 %. HC ≥ 2.1 kOe and MS of 73 emu/g are obtained in the final sintered ceramic magnets, exhibiting the highest HC value of 2.8 kOe for the magnet sintered using glacial acetic acid. 相似文献
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《International Journal of Hydrogen Energy》2022,47(18):10137-10155
In this work, hydrate based separation technique was combined with membrane separation and amine-absorption separation technologies to design hybrid processes for separation of CO2/H2 mixture. Hybrid processes are designed in the presence of different types of hydrate promoters. The conceptual processes have been developed using Aspen HYSYS. Proposed processes were simulated at different flow rates for the feed stream. A comprehensive cost model was developed for economic analysis of novel processes proposed in this study. Based on the results from process simulation and equipment sizing, the amount of total energy consumption, fixed cost, variable cost, and total cost were calculated per unit weight of captured CO2 for various flow rates of feed stream and in the presence of different hydrate promoters. Results showed that combination of hydrate formation separation technique with membrane separation technology results in a CO2 capture process with lowest energy consumption and total cost per unit weight of captured CO2. As split fraction and heat of hydrate formation increases, the share of hydrate formation section in total energy consumption increases. When TBAB is applied as hydrate promoter, due to its higher hydrate separation efficiency, more amount of CO2 is captured in hydrate formation section and consequently the total cost for process decreases considerably. Hybrid hydrate-membrane process in the presence of TBAB as hydrate promoter with 29.47 US$/ton CO2 total cost is the best scheme for hybrid hydrate CO2 capture process. Total cost for this process is lower than total cost for single MDEA-based absorption process as the mature technology for CO2 capture. 相似文献
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《Mechatronics》2022
A large-scale high-precision scan stage is important equipment in the industrial productions of micro-fabrication such as flat panel display (FPD) lithography systems. Designing controllers for multi-input multi-output (MIMO) systems is time-consuming and needs experience because of the interaction between each axis and many controller tuning parameters. The aim of this study is to develop a peak filter design method based on frequency response data to reduce repetitive disturbance. This data-based approach does not use the model and only uses the frequency response data of the controlled system and the disturbance spectrum calculated from the scanning error data (Contribution 1). The peak filter is designed by convex optimization and satisfies robust stability conditions for six-degree-of-freedom systems (Contribution 2). The control performance of the designed peak filter is experimentally demonstrated with an industrial MIMO large-scale high-precision scan stage in reducing the scanning error of the main stroke of the translation along the -axis (Contribution 3). 相似文献
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