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Hydrogen peroxide (H2O2) has been listed as one of the 100 most important chemicals in the world. However, huge amount of residual H2O2 is hard to timely decomposed into O2 and H2O under acidic condition, easily resulting in explosion hazard. Here, we reported a core–shell structure catalyst, that is graphene with Co N structure encapsulated Co nanoparticles. Co N graphene shell serves as the active site for the H2O2 decomposition, and Co core further enhance this decomposition. Benefiting from it, the H2O2 decomposition were close to 100% after 6 cycles without pH adjustment, which increased 6 orders of magnitude compared with no catalyst. At the same time, the O2 generation reached 99.67% in 2 h with little metal leaching, and ·OH has been greatly inhibited to only 0.08%. This work can cleanly remove H2O2 with little deep oxidation and protect the process of H2O2 utilization to achieve a safer world.  相似文献   
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Qin  Yuancheng  Yao  Yingbiao  Feng  Wei  Li  Pei  Xu  Xin 《Wireless Networks》2022,28(8):3337-3347
Wireless Networks - With the dynamic voltage scaling (DVS) technology, the terminal node (TN) can dynamically adjust its computational speed, thus providing a new way to save energy during task...  相似文献   
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Feng  Zilong  Na  Zhenyu  Xiong  Mudi  Ji  Chenglan 《Mobile Networks and Applications》2022,27(4):1578-1592
Mobile Networks and Applications - Due to fast deployment, strong survivability and flexible scheduling, multiple unmanned aerial vehicles (UAV) can synergistically optimize the trajectory and...  相似文献   
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Chen  Huiling  Zhang  Chunmei  Xu  Qin  Feng  Yuli 《Neural Processing Letters》2022,54(1):181-205
Neural Processing Letters - This paper is concerned with topology identification of stochastic multi-weighted complex networks based on adaptive synchronization. Different from previous work,...  相似文献   
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Corrosion and salt deposition problems severely restrict the industrialization of supercritical water oxidation. Transpiring wall reactor can effectively weaken these two problems by a protective water film. In this work, methanol was selected as organic matter, and the influences of vital structural parameters on water film properties and organic matter removal were studied via numerical simulation. The results indicate that higher than 99% of methanol conversion could be obtained and hardly affected by transpiration water layer, transpiring wall porosity and inner diameter. Increasing layer and porosity reduced reactor center temperature, but inner diameter's influence was lower relatively. Water film temperature reduced but coverage rate raised as layer, porosity, and inner diameter increased. Notably, the whole reactor was in supercritical state and coverage rate was only approximately 85% in the case of one layer. Increasing reactor length affected slightly the volume of the upper supercritical zone but enlarged the subcritical zone.  相似文献   
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Fine-grained few-shot learning is a difficult task in image classification. The reason is that the discriminative features of fine-grained images are often located in local areas of the image, while most of the existing few-shotlearning image classification methods only use top-level features and adopt a single measure. In that way, the localfeatures of the sample cannot be learned well. In response to this problem, ensemble relation network with multi-level measure (ERN-MM) is proposed in this paper. It adds the relation modules in the shallow feature space tocompare the similarity between the samples in the local features, and finally integrates the similarity scores from thefeature spaces to assign the label of the query samples. So the proposed method ERN-MM can use local details andglobal information of different grains. Experimental results on different fine-grained datasets show that the proposedmethod achieves good classification performance and also proves its rationality.  相似文献   
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文章分析智能建造技术创新主体的特点,界定并划分智能建造技术协同创新主体互动关系的范畴和类别,建立智能建造协同创新的多方演化博弈模型,揭示智能建造技术协同创新主体互动关系。主要结论为:①智能建造技术协同创新呈现级联性、函数性、动态平衡性、不确定性和指数性特征;②智能建造技术协同创新主体互动关系分为同质性的内部主体互动和异质性的内部主体与外部主体互动,表现出利益共生、成长进化和共享协同的特征;③创新主体之间的互动行为有利于对创新资源进行有效配置,推动智能建造技术的应用。  相似文献   
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