全文获取类型
收费全文 | 1854篇 |
免费 | 82篇 |
国内免费 | 3篇 |
专业分类
电工技术 | 106篇 |
综合类 | 6篇 |
化学工业 | 439篇 |
金属工艺 | 44篇 |
机械仪表 | 51篇 |
建筑科学 | 29篇 |
能源动力 | 81篇 |
轻工业 | 132篇 |
水利工程 | 4篇 |
无线电 | 137篇 |
一般工业技术 | 382篇 |
冶金工业 | 321篇 |
原子能技术 | 70篇 |
自动化技术 | 137篇 |
出版年
2023年 | 11篇 |
2022年 | 5篇 |
2021年 | 18篇 |
2020年 | 17篇 |
2019年 | 18篇 |
2018年 | 50篇 |
2017年 | 41篇 |
2016年 | 42篇 |
2015年 | 28篇 |
2014年 | 40篇 |
2013年 | 90篇 |
2012年 | 89篇 |
2011年 | 118篇 |
2010年 | 87篇 |
2009年 | 58篇 |
2008年 | 92篇 |
2007年 | 96篇 |
2006年 | 67篇 |
2005年 | 69篇 |
2004年 | 51篇 |
2003年 | 53篇 |
2002年 | 46篇 |
2001年 | 28篇 |
2000年 | 27篇 |
1999年 | 41篇 |
1998年 | 129篇 |
1997年 | 85篇 |
1996年 | 58篇 |
1995年 | 41篇 |
1994年 | 30篇 |
1993年 | 41篇 |
1992年 | 21篇 |
1991年 | 29篇 |
1990年 | 14篇 |
1989年 | 21篇 |
1988年 | 19篇 |
1987年 | 19篇 |
1986年 | 11篇 |
1985年 | 13篇 |
1984年 | 15篇 |
1983年 | 9篇 |
1982年 | 16篇 |
1981年 | 21篇 |
1980年 | 5篇 |
1979年 | 13篇 |
1978年 | 10篇 |
1977年 | 12篇 |
1976年 | 13篇 |
1974年 | 3篇 |
1972年 | 4篇 |
排序方式: 共有1939条查询结果,搜索用时 31 毫秒
1.
Hideo Yamauchi Junichi Ikejiri Fumio Sato Hiroyuki Oshita Tsuyoshi Honma Takayuki Komatsu 《Journal of the American Ceramic Society》2019,102(11):6658-6667
In recent years, the expansion of demand for lithium ion batteries has resulted in soaring prices of the constituent resources. From the viewpoint of safety, studies on all-solid-state batteries are actively being carried out. In this study, we succeeded in driving all-solid-state batteries derived from nontoxic oxide glasses at room temperature without requiring scarce resources such as lithium and cobalt. The main structure of the ceramic batteries with a simple structure in which Na2FeP2O7 crystallized glass and β″-alumina solid solution are joined by pressureless cofiring at 550°C. During the crystallization of Na2O-Fe2O3-P2O5 glass, fusion with the β″-alumina solid solution is achieved. Reversible charge and discharge of 80 mAh/g were achieved at room temperature. It is not necessary to apply pressure during cell preparation or the use of the batteries. Furthermore, the strong junction at the cathode and electrolyte interface does not peel off during charge and discharge over a long period of 623 cycles. Ex situ X-ray photoelectron spectroscopy revealed partial Fe4+ induction and a reversible charge and discharge reaction even after overcharging to 9 V. It was demonstrated that Na2FeP2O7 is very stable against overcharging to 9 V. 相似文献
2.
3.
Dr. Takuya Kobayakawa Kento Ebihara Yuzuna Honda Dr. Masayuki Fujino Dr. Wataru Nomura Prof. Naoki Yamamoto Dr. Tsutomu Murakami Prof. Hirokazu Tamamura 《Chembiochem : a European journal of chemical biology》2019,20(16):2101-2108
C34, a 34-mer fragment peptide, is contained in the HIV-1 envelope protein gp41. A dimeric derivative of C34 linked through a disulfide bridge at its C terminus was synthesized and found to display potent anti-HIV activity, comparable with that of a previously reported PEGylated dimer of C34REG. The reduction in the size of the linker moiety for dimerization was thus successful, and this result might shed some light on the mechanism of the suppression of six-helix bundle formation by these C34 dimeric derivatives. Addition of a Gly-Cys(CH2CONH2)-Gly-Gly motif at the N-terminal position of a C34 monomeric derivative significantly increased the anti-HIV-1 activity. This moiety functions as a new pharmacophore, and this might provide a useful insight into the design of potent HIV-1 fusion inhibitors. 相似文献
4.
Akio Ohta Faisal Hossain Hitoshi Asakawa Tsuyoshi Asakawa 《Journal of surfactants and detergents》2020,23(1):99-108
Cysteine and methionine, two sulfur-containing amino acids (AA), were introduced in their surfactant forms as potential antioxidants. The antioxidative (AOX) properties of lauroyl methionine (C12-Met) and lauroyl cysteine (C12-Cys) was investigated by means of the oxygen radical absorbance capacity assay. Both the surfactants exhibited excellent AOX behavior at the premicellar state and micellar medium. The AOX behavior was found to be comparable for both the surfactants at their premicellar states. However, in micellar medium, C12-Met showed better AOX property than C12-Cys. The AOX power of the surfactants was compared with other previously developed AA-type surfactants. The order of the AOX power was found to be: C12-tryptophan > C12-tyrosine ≈ C12-methionine ≈ C12-cysteine > C12-histidine at the premicellar state and C12-tryptophan > C12-tyrosine > C12-methionine > C12-cysteine > C12-histidine at the micellar state. C12-Cys displayed lower AOX property in micellar medium due to its dimer formation tendency. Based on the HPLC and UPLC-Q-TOF-MS analysis, the dimer formation of C12-Cys was found to be accelerated due to the micellar environment and results into negative synergistic effect on other aromatic AA-type surfactants. However, the presence of C12-His in the micellar solution of C12-Cys resulted no synergistic effect due to stronger H-bonding between the surfactants and resulting less dimer formation. 相似文献
5.
Current Control Method of Achieving Wide‐Range Power Driving for Linear Synchronous Motor with Half‐Wave‐Rectified Self‐Excitation 下载免费PDF全文
In a previous paper, we proposed a novel linear synchronous motor with half‐wave‐rectified self‐excitation. A long‐stator‐type linear synchronous motor was built and its performance was verified by experiments. This paper presents a new current control method for the linear synchronous motor in order to achieve a wide range of speeds and high‐power operations. First, we propose a current control method for high‐thrust operation in the constant‐thrust region. This operation is realized by using the reluctance thrust resulting from the saliency of the linear synchronous motor. We also propose a control method that maximizes the ratio of the thrust to the voltage; this method can be used to expand the operating range. Wide‐range‐speed operation can be achieved by applying this new control method along with field‐weakening control. The thrust and operating characteristics of the proposed control methods are estimated by performing experiments and coupled electric and magnetic analysis. 相似文献
6.
Shahira Said Aly Tsuyoshi Imai Mohamed Salah Hassouna Diem-Mai Kim Nguyen Takaya Higuchi Ariyo Kanno Koichi Yamamoto Rinji Akada Masahiko Sekine 《International Journal of Hydrogen Energy》2018,43(10):5300-5313
The ability of Clostridium butyricum RAK25832 to use casamino acids as a nitrogen source was investigated. Strain RAK25832 showed the capacity to utilize different types of carbon sources. With glucose as a carbon source (10 g/L), the preferred final concentration of casamino acids was 26.67 g/L, with a cumulative hydrogen production, production rate, and yield of 2505 mL H2/L, 160 mL/h, and 1.81 mol H2/mol glucose, respectively. Eighteen metal elements were screened to identify the most important metals for biohydrogen production, and four elements were optimized. The optimal medium composition was MgCl2·6H2O (0.1 g/L), K2HPO4·3H2O (6.67 g/L), NaHCO3 (2.6 g/L), and FeCl2·4H2O (0.002 g/L). Vitamin supplementation of the medium showed no significant effect on hydrogen production. Under the optimized conditions, cumulative hydrogen production reached 3074 mL H2/L. This is the first study to demonstrate the use of casamino acids as a nitrogen source by C. butyricum. 相似文献
7.
Koutaki Gou Ando Sakino Shirai Keiichiro Kishigami Tsuyoshi 《International Journal of Computer Vision》2022,130(9):2286-2304
International Journal of Computer Vision - In April 2016, a massive earthquake with a magnitude of 7.3 struck Kumamoto region, Japan, causing major devastation. One of the structures that were... 相似文献
8.
Reed (Phragmites australis), a commonly used macrophyte in the wetlands constructed for water purification, was investigated as a new biosorbent for the removal of Cu(2+), Cd(2+), Ni(2+), Pb(2+) and Zn(2+) from aqueous solution. The metal adsorption capacity of reed biomass was improved significantly by water-wash, base- and acid-treatment. The maximum sorption of NaOH-pretreated reed biomass was observed near neutral pH for Cu(2+), Cd(2+), Ni(2+) and Zn(2+), while that for Pb(2+) was from an acidic range of pH 4.0 or higher. The maximum metal adsorption capacity on a molar basis assumed by Langmuir model was in the order of Cu(2+)>Ni(2+)>Cd(2+)>Zn(2+)>Pb(2+). Reed biosorbent showed a very high adsorption affinity value, which helps predict its high ability to adsorb heavy metals at low concentration. Desorption of heavy metals and regeneration of the biosorbent was attained simultaneously by acid elution. Even after three cycles of adsorption-elution, the adsorption capacity was regained completely and the desorption efficiency of metal was maintained at around 90%. 相似文献
9.
Kunihiro Ogata Tokio Umino Tsuyoshi Nakayama Eiichi Ono Toshiaki Tsuji 《Advanced Robotics》2017,31(6):303-310
Development of clothing in consideration of the shape and body function of a person with spinal cord injury is an important task. Then, a dummy robot with a deformation mechanism was developed in this study for evaluating the comfortable level of clothings. Specifically, a trunk joint mechanism and an abdominal mechanism that can realize various deformations of the abdominal area and various trunk poses were developed. The trunk joint mechanism was implemented in order to simulate the seated posture of persons with spinal cord injury. The abdominal deformation mechanism was implemented using linear actuators and rotating servomotors in order to simulate abdominal obesity of persons with spinal cord injury. Further, a tactile sensor system was developed for measuring the clothing pressure on the abdominal area and evaluating the comfort or discomfort of clothing. 相似文献
10.
Effect of annealing on photovoltaic properties and microstructure of conventional and inverted organic solar cells using active bilayer based on liquid‐crystal semiconducting polymer and fullerene 下载免费PDF全文
Atsushi Suzuki Hisato Suzuki Haruto Maruhashi Syoto Banya Tsuyoshi Akiyama Takeo Oku 《国际能源研究杂志》2014,38(12):1541-1550
Conventional and inverted organic solar cells of poly[9,9‐dioctyl‐fluorene‐co‐bithiophene] (F8T2) as liquid‐crystal semiconducting polymer and fullerene as electron acceptor were fabricated and characterized. An effect of thermal treatment of the films on annealing condition near glass transition was investigated for tuning optimization and improving the photovoltaic and optical properties. Annealing treatment below the glass transition improved the photovoltaic performance and carrier diffusion in crystal growth of active layer. The X‐ray diffraction patterns indicate a crystalline structure with molecular order of F8T2 in crystal index, 100 as a layer distance between sheets of F8T2 chains. The photovoltaic properties were based on molecular interactions with molecular ordering in active layer at crystal state. As the photovoltaic mechanisms, the F8T2 thin film as p‐type semiconducting polymer worked for electron‐donor layer to support light‐induced generation, carrier diffusion and charge transfer near interface in active layer. Copyright © 2014 John Wiley & Sons, Ltd. 相似文献